High-Temperature Short-Time Treated Polylactic Acid Pleated Hydrocharged Melt Blown Nonwoven with Enhanced Charge Storage Capacity

IF 4.4 2区 化学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY
Yixuan Chen, Qiwei Huang, Yanyan Lin, Bin Ding, Jianyong Yu, Hong Wang* and Xianfeng Wang*, 
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Abstract

Biodegradable filter materials with high filtration effectiveness is essential for safeguarding human health. This study focused on the melt blown nonwoven fabric composed of polylactic acid and polycaprolactone as raw materials, with nanosilica serving as the electret material. In contrast to smooth fibers, the pleated fibers was subjected to a high temperature, short-time heat-setting method. Ultimately, sophisticated hydrocharging technology is employed to electret the processed nonwoven material, pleated fibers produce and retain a significant electrical charge following the hydrocharging process. The charge production capacity has been augmented nearly 2-fold (from 199 V to 598 V), and the storage capacity has been significantly enhanced (from 1.45 pA to 2.08 pA). The nonwoven fabric exhibits exceptional filtration efficiency (98.05 ± 0.18%), minimal pressure decreases (60.76 ± 0.05 Pa), and a commendable quality factor (0.16 Pa–1). It is noteworthy that, following the evaluation of the crystallization capability, surface electrostatic potential, and charge storage characteristics of the self-fabricated nonwoven fabric, we have systematically elucidated the mechanisms of pleat formation and charge storage, thereby providing theoretical guidance for the development of future pleated filtration materials.

高温短时处理聚乳酸褶皱加氢熔喷非织造布增强电荷储存能力
具有高过滤效率的生物可降解过滤材料是保障人体健康必不可少的。研究了以聚乳酸和聚己内酯为原料,纳米二氧化硅为驻极体材料的熔喷非织造布。与光滑纤维相比,褶皱纤维经受了高温、短时间热定型方法。最后,采用复杂的充氢技术对加工过的非织造材料进行驻极体化,褶皱纤维在充氢过程中产生并保留大量电荷。电荷生产能力提高了近2倍(从199 V提高到598 V),存储容量显著提高(从1.45 pA提高到2.08 pA)。该非织造布具有优异的过滤效率(98.05±0.18%)、最小压力降低(60.76±0.05 Pa)和优良的品质系数(0.16 Pa - 1)。值得注意的是,在对自制非织造布的结晶能力、表面静电势、电荷存储特性进行评价的基础上,系统地阐明了褶皱形成和电荷存储的机理,从而为未来褶皱过滤材料的开发提供理论指导。
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来源期刊
CiteScore
7.20
自引率
6.00%
发文量
810
期刊介绍: ACS Applied Polymer Materials is an interdisciplinary journal publishing original research covering all aspects of engineering, chemistry, physics, and biology relevant to applications of polymers. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrates fundamental knowledge in the areas of materials, engineering, physics, bioscience, polymer science and chemistry into important polymer applications. The journal is specifically interested in work that addresses relationships among structure, processing, morphology, chemistry, properties, and function as well as work that provide insights into mechanisms critical to the performance of the polymer for applications.
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