Regulation of surface carbon dioxide distributions and air–sea fluxes by temperature, biology, and mixing along the North American Atlantic Coastal Ocean Margin

IF 3.8 1区 地球科学 Q1 LIMNOLOGY
Zelun Wu, Xinyu Li, Zhangxian Ouyang, Wei‐Jun Cai
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Abstract

The North American Atlantic Coastal Ocean Margin (NAACOM) was recognized as an atmospheric carbon dioxide (CO2) sink, with large uncertainties in its northern areas due to complex dynamics in controlling the spatiotemporal variability of surface partial pressure of CO2 (pCO2) and limited pCO2 observations. Here, we used a regional reconstructed product to investigate the spatial and seasonal variability of pCO2 and air–sea CO2 fluxes across the region during 1993–2021. Decomposition of pCO2 variability reveals temperature as the primary driver in southern sub‐regions (Gulf of Mexico, South and Mid Atlantic Bight), while both thermal and nonthermal processes dominate in the north (Gulf of Maine, Scotian Shelf, Gulf of St. Lawrence, and Grand Banks), with winter deep mixing leading to pCO2 elevation, and spring phytoplankton production significantly influencing pCO2 drawdown. These regional differences in local dynamics result in greater air–sea CO2 disequilibrium in the north, driving larger seasonal pCO2 amplitudes, and a pronounced south‐to‐north decreasing gradient. We identified the entire region as a CO2 sink, with fluxes of −0.63 ± 0.19 and −0.60 ± 0.21 mol C m−2 yr−1 (10.14 ± 3.00 and 24.24 ± 8.31 Tg C yr−1), respectively, in the narrow (depth < 200 m) and wide (distance from shoreline < 400 km) ocean margins. The updated wide‐margin CO2 uptake is 61% lower than previous reports. This 29‐yr analysis elucidates the drivers of pCO2 variability across the diverse NAACOM, highlighting the importance of regional pCO2 products for improving coastal carbon systems projections in a changing climate.
温度、生物和北美大西洋沿岸海洋边缘混合对表面二氧化碳分布和海气通量的调节
北美大西洋海岸边缘(NAACOM)被认为是一个大气二氧化碳(CO2)汇,其北部地区由于控制地表CO2分压(pCO2)时空变化的复杂动力学和有限的pCO2观测值,存在较大的不确定性。利用区域重建产品研究了1993-2021年该区域pCO2和海气CO2通量的空间和季节变化。对pCO2变率的分解表明,温度是南部次区域(墨西哥湾、南大西洋和中大西洋湾)的主要驱动因素,而北部次区域(缅因湾、斯科斯大陆架、圣劳伦斯湾和大浅滩)的热和非热过程占主导地位,冬季深层混合导致pCO2升高,春季浮游植物生产显著影响pCO2降低。这些局部动力的区域差异导致北部更大的海气CO2不平衡,驱动较大的季节pCO2振幅,以及明显的南向北递减梯度。我们将整个区域确定为CO2汇,在狭窄的(深度和深度)中,通量分别为- 0.63±0.19和- 0.60±0.21 mol C m−2 yr−1(10.14±3.00和24.24±8.31 Tg C yr−1);200米)和宽(距离海岸线<;400公里)的海洋边缘。最新的宽边际二氧化碳吸收量比以前的报告低61%。这一29年的分析阐明了不同NAACOM地区二氧化碳分压变化的驱动因素,强调了区域二氧化碳分压产品在气候变化中改善沿海碳系统预测的重要性。
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来源期刊
Limnology and Oceanography
Limnology and Oceanography 地学-海洋学
CiteScore
8.80
自引率
6.70%
发文量
254
审稿时长
3 months
期刊介绍: Limnology and Oceanography (L&O; print ISSN 0024-3590, online ISSN 1939-5590) publishes original articles, including scholarly reviews, about all aspects of limnology and oceanography. The journal''s unifying theme is the understanding of aquatic systems. Submissions are judged on the originality of their data, interpretations, and ideas, and on the degree to which they can be generalized beyond the particular aquatic system examined. Laboratory and modeling studies must demonstrate relevance to field environments; typically this means that they are bolstered by substantial "real-world" data. Few purely theoretical or purely empirical papers are accepted for review.
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