Evaluation of emissions and spatial distribution of methane from offshore oil and gas platforms in the Liaodong Bay of China based on shipboard measurement†

IF 3.9 3区 环境科学与生态学 Q1 CHEMISTRY, ANALYTICAL
Yue Yu, Zongcai He, Qing Su, Xuemei Xu, Jiayi Cheng, Yue Ming, Xiaomeng Wang, Hong Chen and Jianbo Han
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Abstract

Offshore oil and gas platforms are a notable source of methane (CH4) in the marine environment, yet there remains a lack of comprehensive understanding regarding their impact along the coastal areas of China. Besides, relevant emissions are generally derived from systematic inventory and rarely quantified by top–down methods. To this end, a ship-based measurement of CH4 emissions from three offshore oil and gas platforms with different oil and gas production levels was conducted over the Liaodong Bay of China in August 2023. The results demonstrated that there were differences in CH4 background concentrations around the three platforms (2291 ± 15 ppb, 2468 ± 32 ppb and 2100 ± 12 ppb). At moderate wind speeds, CH4 levels showed a gradual increase as the ship approached the target upwind, with peak concentrations typically observed within a range of 2–3 km from the platform. Along with meteorological data and the Gaussian plume model, CH4 emission rates were determined corresponding to the average values of 229 ± 48 kg h−1, 59 ± 16 kg h−1 and 13 ± 8 kg h−1 for the three platforms. By analyzing the concurrent changes in carbon dioxide concentration, it was hypothesized that gas flaring was the primary source of CH4 emissions from one of the platforms. Additionally, when considering the revised emission factors for the oil and gas industry from the IPCC and combining them with the production data from the three platforms, the results clearly demonstrated a substantial contrast between top–down emissions and inventory emissions. Diverse platforms and continuous monitoring are necessary to validate the aforementioned perspective and ultimately enhance the precision of CH4 emission data provided to regulators and the general public.

Abstract Image

基于船载测量的辽东湾海上油气平台甲烷排放及空间分布评价
海洋油气平台是海洋环境中甲烷(CH4)的重要来源,但对其对中国沿海地区的影响仍缺乏全面的认识。此外,相关排放量一般是通过系统的清查得出的,很少采用自上而下的方法进行量化。为此,于2023年8月在中国辽东湾对三个不同油气生产水平的海上油气平台进行了船舶测量。结果表明,三个平台周围的CH4背景浓度(2291±15 ppb, 2468±32 ppb和2100±12 ppb)存在差异。在中等风速下,CH4水平随着船舶接近逆风目标而逐渐增加,通常在距离平台2-3公里的范围内观察到峰值浓度。结合气象资料和高斯羽流模型,确定了3个平台对应的CH4排放速率平均值为229±48 kg h-1、59±16 kg h-1和13±8 kg h-1。通过分析二氧化碳浓度的同步变化,我们假设天然气燃烧是其中一个平台排放CH4的主要来源。此外,当考虑IPCC修订后的油气行业排放因子,并将其与三个平台的生产数据相结合时,结果清楚地显示了自上而下排放与库存排放之间的巨大差异。为了验证上述观点,最终提高向监管机构和公众提供CH4排放数据的精度,需要多种平台和持续监测。
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来源期刊
Environmental Science: Processes & Impacts
Environmental Science: Processes & Impacts CHEMISTRY, ANALYTICAL-ENVIRONMENTAL SCIENCES
CiteScore
9.50
自引率
3.60%
发文量
202
审稿时长
1 months
期刊介绍: Environmental Science: Processes & Impacts publishes high quality papers in all areas of the environmental chemical sciences, including chemistry of the air, water, soil and sediment. We welcome studies on the environmental fate and effects of anthropogenic and naturally occurring contaminants, both chemical and microbiological, as well as related natural element cycling processes.
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