Percolation-based mean field theory for disordered particle packings

IF 4.5 2区 工程技术 Q2 ENGINEERING, CHEMICAL
Wenxiang Xu , Zhuangwei Ma , Junliang Fu , Yang Jiao
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引用次数: 0

Abstract

Dense disordered packings of hard particles are useful models for granular materials, composites, colloids, foams, and condensed matter. It is very challenging to devise predictive theories of random packings, due to their intrinsic non-equilibrium and non-local nature. Here, we develop a mean-field theory for disordered particle packings by exploiting a recently discovered percolation transition of the hard-particle contact network that precedes the jamming transition. Assuming that the salient structural correlations in the final jammed packing are mainly inherited from those emerging in the percolating particle network, we devise a mean-field formalism that maps the hard particle percolation to analytically solvable Bethe-lattice models. This allows us to establish an analytical relation connecting the packing fraction ϕ and average contact number Z for a wide spectrum of congruent non-spherical hard particles in three-dimensional Euclidean space 3, where the particle shape factor is rescaled by the percolation critical exponent, reflecting the coupling of local and large scales in our mean-field formalism. The accuracy of our theory is ascertained by comparing its predictions of ϕ to the corresponding numerical values reported in literature. Our mean-field theory can be readily generalized to higher dimensions.
无序粒子堆积的基于渗流的平均场理论
硬颗粒的密集无序填料是颗粒材料、复合材料、胶体、泡沫和凝聚态物质的有用模型。由于随机填料本身的非平衡性和非局域性,其预测理论的设计具有很大的挑战性。在这里,我们通过利用最近发现的硬颗粒接触网络在干扰转变之前的渗透转变,发展了无序颗粒堆积的平均场理论。假设最终堵塞填料中的显著结构相关性主要继承于渗透粒子网络中出现的结构相关性,我们设计了一个平均场形式,将硬粒子渗透映射到解析可解的贝特格模型。这使我们能够建立一个解析关系,连接三维欧几里德空间中宽谱全等非球形硬粒子的填充分数φ和平均接触数Z,其中粒子形状因子通过渗透临界指数重新缩放,反映了我们的平均场形式中局部尺度和大尺度的耦合。我们的理论的准确性是通过比较其φ的预测到相应的数值报告在文献中确定的。我们的平均场理论可以很容易地推广到更高的维度。
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来源期刊
Powder Technology
Powder Technology 工程技术-工程:化工
CiteScore
9.90
自引率
15.40%
发文量
1047
审稿时长
46 days
期刊介绍: Powder Technology is an International Journal on the Science and Technology of Wet and Dry Particulate Systems. Powder Technology publishes papers on all aspects of the formation of particles and their characterisation and on the study of systems containing particulate solids. No limitation is imposed on the size of the particles, which may range from nanometre scale, as in pigments or aerosols, to that of mined or quarried materials. The following list of topics is not intended to be comprehensive, but rather to indicate typical subjects which fall within the scope of the journal's interests: Formation and synthesis of particles by precipitation and other methods. Modification of particles by agglomeration, coating, comminution and attrition. Characterisation of the size, shape, surface area, pore structure and strength of particles and agglomerates (including the origins and effects of inter particle forces). Packing, failure, flow and permeability of assemblies of particles. Particle-particle interactions and suspension rheology. Handling and processing operations such as slurry flow, fluidization, pneumatic conveying. Interactions between particles and their environment, including delivery of particulate products to the body. Applications of particle technology in production of pharmaceuticals, chemicals, foods, pigments, structural, and functional materials and in environmental and energy related matters. For materials-oriented contributions we are looking for articles revealing the effect of particle/powder characteristics (size, morphology and composition, in that order) on material performance or functionality and, ideally, comparison to any industrial standard.
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