Slippery liquid infused porous surface coupling with exposed spindle-like hydrophilic-hydrophobic bumps for enhanced atmosphere fog collection

IF 8.3 1区 工程技术 Q1 ENGINEERING, CHEMICAL
Junda Wu, Jiangdong Dai, Chunxiang Li, Jianming Pan, Yongsheng Yan
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Abstract

Water collection on slippery liquid infused porous surface (SLIPS) is commonly effective due to the brilliant water transportation and removal property. However, the limited fog deposition sites on SLIPS results in the low fog capture efficiency in the initial water collection state, mitigates the whole water collection rate (WCR). Herein, the deacetylated cellulose acetate (CH) with unique underoil superhydrophilicity and strong water affinity was as the strong hydrophilic bumps to introduce onto the SLIPS, resolved the issue of incompatibility between hydrophobic SLIPS and hydrophilic bumps, and enhanced the fog capture ability of the surface. Furthermore, the spider silk-like PVDF fibrous was also constructed onto SLIPS to enhance the water droplets coalescence property via endowing unique Laplace pressure. The obtained modified SLIPS performed excellent WCR at around 1581.07 mg cm−2 h−1, which was 48.7 % higher than the original simple SLIPS. This bioinspired surface engineering paradigm establishes systematic quantification of structure-performance correlations in fog harvesting systems, while demonstrating critical design principles for advancing next-generation bioinspired collectors.
光滑的液体注入多孔表面与暴露的纺锤状亲疏水凸起耦合,以增强大气雾收集
由于滑溜液体注入多孔表面(SLIPS)出色的输水和除水性能,其水收集通常是有效的。然而,由于slip上的雾沉降点有限,导致初始集水状态下雾捕获效率较低,降低了整体集水率(WCR)。本文将具有独特的油底超亲水性和强亲水性的去乙酰化醋酸纤维素(CH)作为强亲水突引入到slip上,解决了疏水slip与亲水突不相容的问题,增强了表面的捕雾能力。此外,还将蛛丝状的PVDF纤维构建在slip上,通过赋予独特的拉普拉斯压力来增强水滴的聚并性能。得到的改性SLIPS具有优良的WCR, WCR约为1581.07 mg cm−2 h−1,比原始的简单SLIPS高48.7%。这种受生物启发的表面工程范例建立了雾收集系统中结构-性能相关性的系统量化,同时展示了推进下一代生物启发收集器的关键设计原则。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Desalination
Desalination 工程技术-工程:化工
CiteScore
14.60
自引率
20.20%
发文量
619
审稿时长
41 days
期刊介绍: Desalination is a scholarly journal that focuses on the field of desalination materials, processes, and associated technologies. It encompasses a wide range of disciplines and aims to publish exceptional papers in this area. The journal invites submissions that explicitly revolve around water desalting and its applications to various sources such as seawater, groundwater, and wastewater. It particularly encourages research on diverse desalination methods including thermal, membrane, sorption, and hybrid processes. By providing a platform for innovative studies, Desalination aims to advance the understanding and development of desalination technologies, promoting sustainable solutions for water scarcity challenges.
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