Sponge-Inspired Porous Sensor for Wide-Spectrum Detection of Organic Liquids, Gases, and Isomers.

IF 10.7 2区 材料科学 Q1 CHEMISTRY, PHYSICAL
Chunyi Hu, Qiang Sun, Hongyi Liu, Qiang Zhou, Fandong Meng, Yongyuan Ren, Zhekun Shi, Xiaoli Zhan, Quan Liu, Qinghua Zhang
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引用次数: 0

Abstract

Currently, the identification of organics, including gases, liquids, and isomers, relies heavily on sophisticated analytical equipment or meticulously crafted yet costly materials such as COFs and MOFs. Consequently, developing a straightforward strategy to accurately identify organic gases, liquids, and isomers simultaneously presents a significant challenge. Inspired by the porous structure of the sponge that allows it to absorb multiple liquids quickly, a broad-spectrum micro-nano porous-structure sensor (BPS) is designed using polydimethylsiloxane (PDMS), highly conductive nanoparticle carbon black (CB) and micron-sized thermal expansion microspheres (EM), which utilizes the micro-nano porous structure to enhance the unique swelling interaction between PDMS and various organic compounds, to accurately identify organic gas/liquids, isomers, aqueous solutions, mixed liquids, and even perform quantitative analysis. There are no reports of sensors, such as BPS, capable of simultaneously detecting multiple types of organic matter. The BPS also demonstrates robust performance, retaining its self-cleaning property even after soaking in water, acids, and alkalis. The wide spectrum and high sensitivity of BPS in detecting and identifying volatile organic molecules make it have great potential in the chemical industry, coal, transportation, and other fields.

用于有机液体,气体和异构体宽光谱检测的海绵启发多孔传感器。
目前,有机物(包括气体、液体和异构体)的鉴定在很大程度上依赖于复杂的分析设备或精心制作但昂贵的材料,如COFs和mof。因此,开发一种直接的策略来准确地同时识别有机气体、液体和异构体是一项重大挑战。受海绵可快速吸收多种液体的多孔结构的启发,采用聚二甲基硅氧烷(PDMS)、高导电性纳米颗粒炭黑(CB)和微米级热膨胀微球(EM)设计了一种广谱微纳多孔结构传感器(BPS),利用微纳多孔结构增强PDMS与各种有机化合物之间独特的溶胀相互作用,准确识别有机气体/液体、异构体、水溶液,混合液体,甚至进行定量分析。目前还没有类似BPS的传感器能够同时检测多种有机物质的报道。BPS也表现出了强大的性能,即使浸泡在水、酸和碱中,也能保持其自清洁性能。BPS在检测和鉴定挥发性有机分子方面的广谱性和高灵敏度使其在化工、煤炭、交通运输等领域具有很大的应用潜力。
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来源期刊
Small Methods
Small Methods Materials Science-General Materials Science
CiteScore
17.40
自引率
1.60%
发文量
347
期刊介绍: Small Methods is a multidisciplinary journal that publishes groundbreaking research on methods relevant to nano- and microscale research. It welcomes contributions from the fields of materials science, biomedical science, chemistry, and physics, showcasing the latest advancements in experimental techniques. With a notable 2022 Impact Factor of 12.4 (Journal Citation Reports, Clarivate Analytics, 2023), Small Methods is recognized for its significant impact on the scientific community. The online ISSN for Small Methods is 2366-9608.
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