Advances on modification of photocatalyst for degradation/removal of organic pollutants from water

Solomon Oluwaseun Akinnawo, Thompson Faraday Ediagbonya
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Abstract

Modification strategies such as surface doping, surface defect engineering, surface sensitization and heterojunction have proved to be highly effective in improving the performance of a photocatalyst towards the degradation removal of organic pollutants from water. Photocatalysts such as N-doped TiO2 nanotubes and S-doped TiO2 nanoparticles prepared via surface doping have been described to displayed higher photocatalytic degradation of methyl orange and malachite green compared to unmodified TiO2 nanoparticles. Moreover, AgI/CdS binary composite fabricated via type-II conventional heterojunction strategy has been recounted in obtaining 91 and 94.5 % removal of tetracycline hydrochloride and methyl orange removal from water. Whereas, GQD/ZnO nanowires photocatalyst developed using a direct z-scheme heterostructure strategy has been investigated to yield three times comparably higher degradation of methylene blue than using pure ZnO nanowires. Similar outcomes have been reported with photocatalysts prepared using surface defect engineering and surface sensitization strategies. In comparison to previous studies, this review accentuates the recent advances on the various modification strategies for enhancing photocatalytic performance in removing organic pollutants from wastewater. While recounting the challenges and direction of future studies in palliating these challenges.

Abstract Image

降解/去除水中有机污染物的光催化剂改性研究进展
表面掺杂、表面缺陷工程、表面敏化和异质结等改性策略已被证明是提高光催化剂降解去除水中有机污染物性能的有效方法。通过表面掺杂制备的n掺杂TiO2纳米管和s掺杂TiO2纳米颗粒等光催化剂与未经修饰的TiO2纳米颗粒相比,对甲基橙和孔雀石绿的光催化降解效果更好。此外,通过ii型常规异质结策略制备的AgI/CdS二元复合材料对盐酸四环素和甲基橙的去除率分别为91%和94.5%。然而,使用直接z-图式异质结构策略开发的GQD/ZnO纳米线光催化剂的亚甲基蓝降解率比使用纯ZnO纳米线高3倍。使用表面缺陷工程和表面敏化策略制备的光催化剂也有类似的结果。在此基础上,综述了近年来提高光催化去除废水中有机污染物性能的各种改性策略的研究进展。同时叙述了应对这些挑战的挑战和未来研究的方向。
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