Kern-Schale-Katalysatorpellets: Das Gelbe vom Ei für den lastflexiblen Festbett-Reaktorbetrieb? Core-Shell Catalyst Pellets: The Egg Yolk for Load-Flexible Reactor Operation?

IF 1.5 4区 工程技术 Q3 ENGINEERING, CHEMICAL
Dr.-Ing. Ronny Tobias Zimmermann, Prof. Dr.-Ing. habil. Kai Sundmacher
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引用次数: 0

Abstract

In the Power-to-X concept, wall-cooled fixed-bed tubular reactors will take on a central role in carrying out exothermic, heterogeneously catalyzed reactions. In order to achieve high product yields without overheating the reactors, effective heat management is required, especially for load-flexible operation. One solution for this is the use of core-shell catalyst pellets. In core-shell catalyst pellets, the catalytically active material is separated from the gas bulk by an inert shell (e.g. ‘egg white’ or ‘egg yolk’ pellets). The advantages and disadvantages of this concept are discussed in this article on the basis of analytical equations as well as experimental results on the laboratory and pilot scales, and compared with other concepts.

Abstract Image

核壳催化转化器颗粒:灵活负载的固定床反应堆运行的蛋黄?核壳催化剂颗粒:装载柔性反应堆操作的蛋黄?
在Power-to-X概念中,壁冷固定床管式反应器将在进行放热、多相催化反应中发挥核心作用。为了在不使反应器过热的情况下实现高产品产量,需要有效的热管理,特别是对于负载灵活的操作。一种解决方案是使用核壳催化剂颗粒。在核壳型催化剂颗粒中,催化活性物质通过惰性壳(例如“蛋清”或“蛋黄”颗粒)与气体体分离。本文根据解析方程以及实验室和中试规模的实验结果,讨论了该概念的优缺点,并与其他概念进行了比较。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Chemie Ingenieur Technik
Chemie Ingenieur Technik 工程技术-工程:化工
CiteScore
3.40
自引率
15.80%
发文量
601
审稿时长
3-6 weeks
期刊介绍: Die Chemie Ingenieur Technik ist die wohl angesehenste deutschsprachige Zeitschrift für Verfahrensingenieure, technische Chemiker, Apparatebauer und Biotechnologen. Als Fachorgan von DECHEMA, GDCh und VDI-GVC gilt sie als das unverzichtbare Forum für den Erfahrungsaustausch zwischen Forschern und Anwendern aus Industrie, Forschung und Entwicklung. Wissenschaftlicher Fortschritt und Praxisnähe: Eine Kombination, die es nur in der CIT gibt!
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