In-situ investigation of real-world emissions from 111 measurements on solid fuel household boilers

IF 8 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES
František Hopan , Martin Chmelář , Jiří Kremer , Milan Dej , Michal Vojtíšek-Lom , Estela D. Vicente , Jiří Ryšavý , Kamil Krpec , Lenka Kuboňová , Alexandr Molčanov , Manuel Schwabl , Jiří Horák
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Abstract

Over the years, emissions from significant stationary and mobile sources have significantly reduced, while solid fuel household combustion appliances have substantially contributed to air pollution. Growing evidence links residential solid fuel combustion to air pollution, prompting extensive studies on emissions. Field-based emission measurements provide more accurate characterisation of real-world emissions. A mobile emissions laboratory and measurement procedure was constructed to measure emissions from domestic boilers in the field, in residential settings, during real-world operation by homeowners using typical fuels. Emissions of total suspended particulate matter (TSP), organic gaseous compounds (OGC), carbon monoxide (CO) and overall thermal efficiency during three-hour operating tests were measured. Data were collected from 111 measurements of boilers, including overfire, downdraft, gasification, and automatic boilers that combust wood pellets, wood chips, wood logs, and coals, covering different brands, constructions, and emissions certification standards. The results show that the investigated newer boilers had lower emissions of CO, OGC, and TSP (approximately half) compared to older boiler technology, resulting in a substantial improvement. The emissions from most of the new boilers were substantially higher (about five times) than their strict applicable limit values due to improper operation. In many cases, fuel size, composition, wood moisture content, boiler installation and maintenance, operating procedure, and operator technical knowledge were considered substandard, with some observations of excessive wear and tampering. The findings confirm the importance of real-world local heating emissions measurements and suggest that relatively fast, inexpensive, and substantial emissions reductions may be achieved by improving the maintenance and education of operators.

Abstract Image

对111个固体燃料家用锅炉实际排放测量的现场调查
多年来,大量固定和移动源的排放已大大减少,而固体燃料家用燃烧器具则大大造成了空气污染。越来越多的证据表明,住宅固体燃料燃烧与空气污染有关,这促使人们对排放进行了广泛的研究。基于现场的排放测量提供了更准确的真实世界排放特征。建立了一个移动排放实验室和测量程序,以测量实际使用典型燃料的房主在现场、在住宅环境中使用的家用锅炉的排放。在三个小时的运行测试中,测量了总悬浮颗粒物(TSP)、有机气体化合物(OGC)、一氧化碳(CO)和总热效率。数据收集自111个锅炉的测量数据,包括过火、下沉、气化和燃烧木屑颗粒、木屑、原木和煤炭的自动锅炉,涵盖不同的品牌、结构和排放认证标准。结果表明,与旧锅炉技术相比,所研究的新锅炉的CO, OGC和TSP排放量较低(约一半),从而实现了实质性的改进。由于操作不当,大部分新锅炉的排放量远高于其严格适用的限值(约五倍)。在许多情况下,燃料尺寸、成分、木材含水率、锅炉安装和维护、操作程序以及操作员的技术知识都被认为是不合格的,还有一些观察结果是过度磨损和篡改。研究结果证实了真实世界局部供暖排放测量的重要性,并建议通过改进操作人员的维护和教育,可以实现相对快速、廉价和大量的减排。
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来源期刊
Science of the Total Environment
Science of the Total Environment 环境科学-环境科学
CiteScore
17.60
自引率
10.20%
发文量
8726
审稿时长
2.4 months
期刊介绍: The Science of the Total Environment is an international journal dedicated to scientific research on the environment and its interaction with humanity. It covers a wide range of disciplines and seeks to publish innovative, hypothesis-driven, and impactful research that explores the entire environment, including the atmosphere, lithosphere, hydrosphere, biosphere, and anthroposphere. The journal's updated Aims & Scope emphasizes the importance of interdisciplinary environmental research with broad impact. Priority is given to studies that advance fundamental understanding and explore the interconnectedness of multiple environmental spheres. Field studies are preferred, while laboratory experiments must demonstrate significant methodological advancements or mechanistic insights with direct relevance to the environment.
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