{"title":"NORM detection challenges in the Gas industry: 3D simulation of Pb-210 presence in Gas field pipework","authors":"D.A. Bradley , A. Taheri","doi":"10.1016/j.radphyschem.2025.112901","DOIUrl":null,"url":null,"abstract":"<div><div>Present interest concerns 3D simulations of the presence of naturally occurring radioactive material (NORM) internal to gas-field pipework. The particular aim is to develop capability for examining <sup>210</sup>Pb NORM in tubulars, valves, other such component parts, separators and storage vessels. To-date the major emphasis of related studies has been on developing best practice for protection of workers dealing with the build-up of NORM-affected facilities, including attachments to inner surfaces of gas piping. Nonetheless, to-date identification and potential environmental impact of thin (few millimetre thick and less) deposits in gas lines has remained challenging. Given an increasing trend in decommissioning activities, in part with industry setting targets for carbon reduction, validation of NORM removal towards obtaining NORM-free piping is a matter of particular interest. Efficacious techniques for removal of internal surface NORM contamination can be expected to increase prospects for reuse and repurposing of NORM-free steel, important in seeking to reduce new steel production and hence reduction of carbon load to the environment. To-date, surveys of the presence of NORM have been dominated by hand-held survey meters, sensing gamma emissions transmitted through affected pipework. To a lesser extent this has been supported by workover samples collections and gamma spectroscopy, examples of which have been covered elsewhere. Herein, the focus is on simulations of the presence of <sup>210</sup>Pb and its progeny, with use made of the TOPAS Monte Carlo code to model the 3D distribution of the electron-, photon- and alpha fluence in- and around small sections of <sup>210</sup>Pb depositions in carbon-steel gas pipes, limited in extent for practical purpose to 10 cm simulated length. Results support the conventional understanding of the low likelihood of sensing the presence of <sup>210</sup>Pb via measurements conducted externally to affected pipes, also highlighting the geometric basis for the propensity for NORM accumulation around pipework bends. Present simulations are intended to help inform development of appropriate detector technology and their use in internal surveys, the various distributions pointing to progressive reduction in detection capability as a function of separation of a sensor from pipe surfaces, radically so for alpha activity as expected. Given the presently assumed conditions, beta particle emission is seen to offer the greatest potential for effective detection. Safe, real-time means for internal surfaces radiometry, are currently under development, doped glass fibres for instance allowing access to pipes of restricted dimensions, including around curvatures. Beta- and gamma-emission detection are the favoured options, with efforts aimed at sensing alpha-particle decay of <sup>210</sup>Po pending characterization of thin sensor coatings.</div></div>","PeriodicalId":20861,"journal":{"name":"Radiation Physics and Chemistry","volume":"235 ","pages":"Article 112901"},"PeriodicalIF":2.8000,"publicationDate":"2025-05-03","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Radiation Physics and Chemistry","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0969806X25003937","RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
Present interest concerns 3D simulations of the presence of naturally occurring radioactive material (NORM) internal to gas-field pipework. The particular aim is to develop capability for examining 210Pb NORM in tubulars, valves, other such component parts, separators and storage vessels. To-date the major emphasis of related studies has been on developing best practice for protection of workers dealing with the build-up of NORM-affected facilities, including attachments to inner surfaces of gas piping. Nonetheless, to-date identification and potential environmental impact of thin (few millimetre thick and less) deposits in gas lines has remained challenging. Given an increasing trend in decommissioning activities, in part with industry setting targets for carbon reduction, validation of NORM removal towards obtaining NORM-free piping is a matter of particular interest. Efficacious techniques for removal of internal surface NORM contamination can be expected to increase prospects for reuse and repurposing of NORM-free steel, important in seeking to reduce new steel production and hence reduction of carbon load to the environment. To-date, surveys of the presence of NORM have been dominated by hand-held survey meters, sensing gamma emissions transmitted through affected pipework. To a lesser extent this has been supported by workover samples collections and gamma spectroscopy, examples of which have been covered elsewhere. Herein, the focus is on simulations of the presence of 210Pb and its progeny, with use made of the TOPAS Monte Carlo code to model the 3D distribution of the electron-, photon- and alpha fluence in- and around small sections of 210Pb depositions in carbon-steel gas pipes, limited in extent for practical purpose to 10 cm simulated length. Results support the conventional understanding of the low likelihood of sensing the presence of 210Pb via measurements conducted externally to affected pipes, also highlighting the geometric basis for the propensity for NORM accumulation around pipework bends. Present simulations are intended to help inform development of appropriate detector technology and their use in internal surveys, the various distributions pointing to progressive reduction in detection capability as a function of separation of a sensor from pipe surfaces, radically so for alpha activity as expected. Given the presently assumed conditions, beta particle emission is seen to offer the greatest potential for effective detection. Safe, real-time means for internal surfaces radiometry, are currently under development, doped glass fibres for instance allowing access to pipes of restricted dimensions, including around curvatures. Beta- and gamma-emission detection are the favoured options, with efforts aimed at sensing alpha-particle decay of 210Po pending characterization of thin sensor coatings.
期刊介绍:
Radiation Physics and Chemistry is a multidisciplinary journal that provides a medium for publication of substantial and original papers, reviews, and short communications which focus on research and developments involving ionizing radiation in radiation physics, radiation chemistry and radiation processing.
The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria. This could include papers that are very similar to previous publications, only with changed target substrates, employed materials, analyzed sites and experimental methods, report results without presenting new insights and/or hypothesis testing, or do not focus on the radiation effects.