{"title":"Synthesis of high-aspect ratio Fe3O4 nanostructures via magnetic field guidance: Toward enhanced microwave absorption performance","authors":"Wuyi Chai, Wei Ding, Mianke Chen, Yikang Qiang, Yiqing Yang, Ruikai Liu, Ganhong Zheng, Zhigao Sheng","doi":"10.1063/5.0265489","DOIUrl":null,"url":null,"abstract":"One-dimensional materials have extensive applications in the field of functional materials, but the preparation of one-dimensional materials with large aspect ratio remains a challenge. Herein, we demonstrate a single-step magnetic field-assisted hydrothermal approach for synthesizing single-crystalline Fe3O4 nanochains with an exceptional aspect ratio of ∼540:1. Systematic investigations reveal that the magnetic field critically regulates the morphology, crystallinity, growth mode, and magnetic properties of Fe3O4, and its excellent microwave absorption performance. The minimum reflection loss for the 1 T single-crystal chain structure reached −61.94 dB at 8.65 GHz (thickness: 3.56 mm), which is approximately 3.4 times greater than that of the zero-field polycrystalline samples. This research provides a feasible solution for low-cost and large-scale synthesis of 1D Fe3O4 nanostructure with high aspect ratio and offers a practical path for optimizing the performance of microwave absorbing materials.","PeriodicalId":8094,"journal":{"name":"Applied Physics Letters","volume":"28 1","pages":""},"PeriodicalIF":3.5000,"publicationDate":"2025-05-02","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Applied Physics Letters","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1063/5.0265489","RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"PHYSICS, APPLIED","Score":null,"Total":0}
引用次数: 0
Abstract
One-dimensional materials have extensive applications in the field of functional materials, but the preparation of one-dimensional materials with large aspect ratio remains a challenge. Herein, we demonstrate a single-step magnetic field-assisted hydrothermal approach for synthesizing single-crystalline Fe3O4 nanochains with an exceptional aspect ratio of ∼540:1. Systematic investigations reveal that the magnetic field critically regulates the morphology, crystallinity, growth mode, and magnetic properties of Fe3O4, and its excellent microwave absorption performance. The minimum reflection loss for the 1 T single-crystal chain structure reached −61.94 dB at 8.65 GHz (thickness: 3.56 mm), which is approximately 3.4 times greater than that of the zero-field polycrystalline samples. This research provides a feasible solution for low-cost and large-scale synthesis of 1D Fe3O4 nanostructure with high aspect ratio and offers a practical path for optimizing the performance of microwave absorbing materials.
期刊介绍:
Applied Physics Letters (APL) features concise, up-to-date reports on significant new findings in applied physics. Emphasizing rapid dissemination of key data and new physical insights, APL offers prompt publication of new experimental and theoretical papers reporting applications of physics phenomena to all branches of science, engineering, and modern technology.
In addition to regular articles, the journal also publishes invited Fast Track, Perspectives, and in-depth Editorials which report on cutting-edge areas in applied physics.
APL Perspectives are forward-looking invited letters which highlight recent developments or discoveries. Emphasis is placed on very recent developments, potentially disruptive technologies, open questions and possible solutions. They also include a mini-roadmap detailing where the community should direct efforts in order for the phenomena to be viable for application and the challenges associated with meeting that performance threshold. Perspectives are characterized by personal viewpoints and opinions of recognized experts in the field.
Fast Track articles are invited original research articles that report results that are particularly novel and important or provide a significant advancement in an emerging field. Because of the urgency and scientific importance of the work, the peer review process is accelerated. If, during the review process, it becomes apparent that the paper does not meet the Fast Track criterion, it is returned to a normal track.