Stabilization and Chirality Control of Topological Meron Textures in Radially Graded Ferroelectric Materials

IF 9.6 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Le Van Lich, Ha Thi Dang, Dang Thi Hong Hue, Ba-Hieu Vu, Van-Hai Dinh, Trong-Giang Nguyen
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Abstract

Polar Meron textures possess unique electric dipole arrangements and electrical responses, offering potential for advanced technologies. While balancing elastic and electrostatic energies has shown promise in creating these textures, achieving precise control remains an ongoing challenge. Here, we introduce a method for inducing a topological Meron texture through electrostatic energy manipulation via a gradient design in material distribution. A phase diagram for polar textures in radially graded ferroelectric thin films is constructed using phase-field modeling. Our results show the stabilization of Meron textures, which geometrically and topologically distinguish from conventional vortex structures. This Meron state is characterized by out-of-plane polarization and toroidal moments, which are tunable with electric fields. A curled electric field can switch the Meron handedness, while homogeneous fields can modify both handedness and chirality. These insights into topological configurations in ferroelectric materials could drive further exploration and innovative applications in next-generation device technologies.

Abstract Image

径向梯度铁电材料中拓扑介子织构的稳定性和手性控制
极介子结构具有独特的电偶极子排列和电响应,为先进技术提供了潜力。虽然平衡弹性和静电能量在创造这些纹理方面显示出希望,但实现精确控制仍然是一个持续的挑战。在这里,我们介绍了一种通过材料分布的梯度设计,通过静电能量操纵来诱导拓扑梅隆织构的方法。利用相场模型建立了径向梯度铁电薄膜中极性织构的相图。我们的研究结果表明,meon织构具有稳定性,在几何和拓扑结构上区别于传统的涡旋结构。这种墨伦态的特征是面外偏振和环面矩,它们可以随电场调节。卷曲电场可以改变梅龙的手性,而均匀电场可以改变梅龙的手性和手性。这些对铁电材料拓扑结构的见解可以推动下一代器件技术的进一步探索和创新应用。
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来源期刊
Nano Letters
Nano Letters 工程技术-材料科学:综合
CiteScore
16.80
自引率
2.80%
发文量
1182
审稿时长
1.4 months
期刊介绍: Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including: - Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale - Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies - Modeling and simulation of synthetic, assembly, and interaction processes - Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance - Applications of nanoscale materials in living and environmental systems Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.
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