An Optoelectrically Switched, Dual-Mode Neuromorphic Sensor for Transient and Accumulative Gas Detection

IF 18.5 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
Jaewon Shin, Young-Woo Jang, Seung-Han Kang, Jeong-Wan Jo, Jong Wook Shin, Yong-Hoon Kim, Sung Kyu Park, Sung Woon Cho
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引用次数: 0

Abstract

Conventional gas sensors typically focus on detecting transient gases with critical gas concentrations but lack the ability to detect hazards resulting from cumulative gas exposure. Here, the study demonstrates a dual-mode nitrogen dioxide (NO2) gas sensor utilizing carbon nanotube thin-film transistors, which features a transient detection mode for sensitive detection of transient gas inflow and accumulation detection mode for monitoring cumulative gas exposure, offering efficient and compact analysis of both immediate and prolonged NO2 exposure. The proposed sensor is capable of detecting NO2 gas through the charge trapping and detrapping mechanisms of gas molecules. The unique capability to switch between the transient detection and accumulation recognition modes is achieved via the controlled modulation of electrical bias and ultraviolet light. More importantly, the gate-bias adjustment facilitates precise sensitivity control by regulating the device's electrical properties, while the UV exposure promotes efficient desorption of attached gas molecules. These features may pave the way for the development of multifunctional gas sensors that can perform both real-time detection and long-term exposure monitoring of toxic gases in compact device architectures.

Abstract Image

用于瞬态和累积气体检测的光电开关双模神经形态传感器
传统的气体传感器通常专注于检测具有临界气体浓度的瞬态气体,但缺乏检测累积气体暴露造成的危害的能力。本研究展示了一种利用碳纳米管薄膜晶体管的双模式二氧化氮(NO2)气体传感器,该传感器具有瞬态检测模式,用于灵敏检测瞬态气体流入,积累检测模式用于监测累积气体暴露,提供即时和长期二氧化氮暴露的高效紧凑分析。该传感器能够通过气体分子的电荷捕获和脱捕机制检测NO2气体。在瞬态检测和积累识别模式之间切换的独特能力是通过控制电偏压和紫外光的调制来实现的。更重要的是,栅极偏置调节有助于通过调节器件的电性能来精确控制灵敏度,而紫外线照射则促进了附着气体分子的有效解吸。这些特性可能为多功能气体传感器的发展铺平道路,这些传感器可以在紧凑的设备架构中对有毒气体进行实时检测和长期暴露监测。
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来源期刊
Advanced Functional Materials
Advanced Functional Materials 工程技术-材料科学:综合
CiteScore
29.50
自引率
4.20%
发文量
2086
审稿时长
2.1 months
期刊介绍: Firmly established as a top-tier materials science journal, Advanced Functional Materials reports breakthrough research in all aspects of materials science, including nanotechnology, chemistry, physics, and biology every week. Advanced Functional Materials is known for its rapid and fair peer review, quality content, and high impact, making it the first choice of the international materials science community.
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