Polydiacetylene-zinc oxide-zinc(II)-cationic surfactant nanocomposites as colorimetric sensors of various polymers: Effects of solvents and cationic surfactants

IF 5.3 3区材料科学 Q2 MATERIALS SCIENCE, MULTIDISCIPLINARY

Materials Research Bulletin Pub Date : 2025-04-17 DOI:10.1016/j.materresbull.2025.113500

Sasiwan Boonmak , Mohamed Mehawed Abdellatif , Kotohiro Nomura , Rakchart Traiphol , Nisanart Traiphol

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Abstract

Polymer industry plays a crucial role in our lifestyle. Different methods have been used to identify polymers, but they are often costly and time-consuming. One of the uncomplicated and worthwhile methods is chromatic sensor. This study demonstrates polydiacetylene (PDA)-based colorimetric sensors for detecting various polymers such as poly(methyl methacrylate), poly(ethylene succinate), poly(propylene carbonate), and aliphatic polyesters. Preparation of the sensors utilizes simple mixing of PDA/zinc(II) ion/zinc oxide nanocomposites and cationic surfactants in organic solvents. Results show that the structures of organic solvents and cationic surfactants strongly affect the sensitivity to specific polymers. Furthermore, the sensors can distinguish polymers with different functional groups. The colorimetric detection of polymers at different concentrations can be achieved by varying the concentration of cation surfactants. The colorimetric sensors is versatile and low-cost, suitable for real-life applications. Our results provide a new developing path of PDA-based colorimetric sensors for qualitative and semi-quantitative analysis of various polymers.

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聚二乙炔-氧化锌-锌(II)-阳离子表面活性剂纳米复合材料作为各种聚合物比色传感器：溶剂和阳离子表面活性剂的影响

聚合物工业在我们的生活方式中起着至关重要的作用。已经使用了不同的方法来识别聚合物，但它们通常既昂贵又耗时。色度传感器是一种简单而有价值的检测方法。本研究展示了基于聚二乙炔（PDA）的比色传感器，用于检测各种聚合物，如聚（甲基丙烯酸甲酯）、聚（琥珀酸乙烯）、聚（碳酸丙烯酯）和脂肪族聚酯。传感器的制备利用PDA/锌（II）离子/氧化锌纳米复合材料和阳离子表面活性剂在有机溶剂中的简单混合。结果表明，有机溶剂和阳离子表面活性剂的结构对特定聚合物的敏感性有很大影响。此外，传感器可以区分不同官能团的聚合物。不同浓度聚合物的比色检测可以通过改变阳离子表面活性剂的浓度来实现。该比色传感器用途广泛，成本低，适合实际应用。我们的研究结果为各种聚合物的定性和半定量分析提供了一条基于pda的比色传感器的新发展途径。

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来源期刊

Materials Research Bulletin 工程技术-材料科学：综合

CiteScore

9.80

自引率

5.60%

发文量

372

审稿时长

42 days

期刊介绍： Materials Research Bulletin is an international journal reporting high-impact research on processing-structure-property relationships in functional materials and nanomaterials with interesting electronic, magnetic, optical, thermal, mechanical or catalytic properties. Papers purely on thermodynamics or theoretical calculations (e.g., density functional theory) do not fall within the scope of the journal unless they also demonstrate a clear link to physical properties. Topics covered include functional materials (e.g., dielectrics, pyroelectrics, piezoelectrics, ferroelectrics, relaxors, thermoelectrics, etc.); electrochemistry and solid-state ionics (e.g., photovoltaics, batteries, sensors, and fuel cells); nanomaterials, graphene, and nanocomposites; luminescence and photocatalysis; crystal-structure and defect-structure analysis; novel electronics; non-crystalline solids; flexible electronics; protein-material interactions; and polymeric ion-exchange membranes.