Jiwon Seo , Seungho Song , Jangwon Byun , Chaewon Yoon , Taejoon Mo , Younghak Kim , Hansoo Kim , Jung-Yeol Yeom , Beomjun Park
{"title":"Optimal passivation process for improved spectroscopic grade CdMnTeSe single crystals based on chromic acid","authors":"Jiwon Seo , Seungho Song , Jangwon Byun , Chaewon Yoon , Taejoon Mo , Younghak Kim , Hansoo Kim , Jung-Yeol Yeom , Beomjun Park","doi":"10.1016/j.net.2025.103577","DOIUrl":null,"url":null,"abstract":"<div><div>This study explores the effects of novel H<sub>2</sub>CrO<sub>4</sub>-based passivant on Cd<sub>0.95</sub>Mn<sub>0.05</sub>Te<sub>0.98</sub>Se<sub>0.02</sub> (CMTS) detectors. Optimal passivation for 3 min improved spectroscopic performance by addressing surface defects. However, longer passivation led to degradation due to Cr-invasion, as shown by XPS analysis. The use of a virtual Frisch grid further enhanced energy resolution, highlighting the potential of CMTS detectors for high-energy gamma spectroscopy. These findings emphasize the importance of precise passivation control and suggest that improved CMTS fabrication and passivation techniques could advance the development of cost-effective, larger volume CdTe-based detectors for room temperature applications.</div></div>","PeriodicalId":19272,"journal":{"name":"Nuclear Engineering and Technology","volume":"57 8","pages":"Article 103577"},"PeriodicalIF":2.6000,"publicationDate":"2025-03-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nuclear Engineering and Technology","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1738573325001457","RegionNum":3,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"NUCLEAR SCIENCE & TECHNOLOGY","Score":null,"Total":0}
引用次数: 0
Abstract
This study explores the effects of novel H2CrO4-based passivant on Cd0.95Mn0.05Te0.98Se0.02 (CMTS) detectors. Optimal passivation for 3 min improved spectroscopic performance by addressing surface defects. However, longer passivation led to degradation due to Cr-invasion, as shown by XPS analysis. The use of a virtual Frisch grid further enhanced energy resolution, highlighting the potential of CMTS detectors for high-energy gamma spectroscopy. These findings emphasize the importance of precise passivation control and suggest that improved CMTS fabrication and passivation techniques could advance the development of cost-effective, larger volume CdTe-based detectors for room temperature applications.
期刊介绍:
Nuclear Engineering and Technology (NET), an international journal of the Korean Nuclear Society (KNS), publishes peer-reviewed papers on original research, ideas and developments in all areas of the field of nuclear science and technology. NET bimonthly publishes original articles, reviews, and technical notes. The journal is listed in the Science Citation Index Expanded (SCIE) of Thomson Reuters.
NET covers all fields for peaceful utilization of nuclear energy and radiation as follows:
1) Reactor Physics
2) Thermal Hydraulics
3) Nuclear Safety
4) Nuclear I&C
5) Nuclear Physics, Fusion, and Laser Technology
6) Nuclear Fuel Cycle and Radioactive Waste Management
7) Nuclear Fuel and Reactor Materials
8) Radiation Application
9) Radiation Protection
10) Nuclear Structural Analysis and Plant Management & Maintenance
11) Nuclear Policy, Economics, and Human Resource Development