Characterization and Health Risk of PM2.5 Exposure in South Tangerang, Indonesia

IF 2.9 3区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
Rika Wijiyanti*, Syukria Kurniawati, Isroil Samihardjo, Dwi Retnowati, Satriani Aga Pasma, Barito Mulyo Ratmono and Muhayatun Santoso, 
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Abstract

This study focuses on the characterization of fine particulate matter (PM2.5) and the assessment of health risks associated with it. PM2.5 samples were collected in Serpong using the SuperSASS (speciation air sampling system) every 3 days from August to October 2022. The mass concentration of PM2.5 was determined gravimetrically, while black carbon (BC) was measured using a reflectance method. Energy-dispersive X-ray fluorescence (EDXRF) was employed to quantify the elemental composition. Additionally, measurement of the reconstructed mass (RCM) for PM2.5 was conducted to enhance the understanding of PM2.5 composition and its sources. The PM2.5 measurements indicated concentrations ranging from 13.07 to 71.26 μg/m3, with an average concentration of 41.80 ± 0.99 μg/m3. Sulfur (S) and lead (Pb) were identified as the predominant metals, with average concentrations of 2.71 ± 1.24 and 1.42 ± 1.28 μg/m3, respectively. The average RCM for PM2.5 was 49.2 ± 12.2%, comprising 15.2% black carbon, 25.7% sulfate, 1.73% soil, 0.84% sea salt, 1.05% smoke and 4.62% trace elements. The health implications of PM2.5 were assessed using the hazard quotient (HQ) and excess lifetime cancer risk (ELCR) for Pb, Cr and nickel Ni. The HQ and ELCR values for the studied metals were within the safe range. The order of HQ values was Pb > Cr > Ni, while the trend of ELCR values was Cr > Pb > Ni across all age groups. These findings provide reliable information regarding PM2.5 concentration and composition, potential sources of PM2.5 and health effect, thereby contributing to the development of an early warning system for air pollution in Serpong, Indonesia.

Abstract Image

印尼南坦格朗PM2.5暴露的特征和健康风险
本研究的重点是细颗粒物(PM2.5)的特征和与之相关的健康风险评估。从2022年8月至10月,每3天使用SuperSASS(物种形成空气采样系统)在雪邦收集PM2.5样本。PM2.5的质量浓度采用重量法测定,黑碳(BC)采用反射率法测定。能量色散x射线荧光(EDXRF)定量元素组成。此外,还对PM2.5的重构质量(RCM)进行了测量,以加强对PM2.5组成及其来源的了解。PM2.5浓度范围为13.07 ~ 71.26 μg/m3,平均浓度为41.80±0.99 μg/m3。硫(S)和铅(Pb)为优势金属,平均浓度分别为2.71±1.24和1.42±1.28 μg/m3。PM2.5的平均RCM为49.2±12.2%,其中黑碳15.2%,硫酸盐25.7%,土壤1.73%,海盐0.84%,烟雾1.05%,微量元素4.62%。利用铅、铬和镍镍的危害商数(HQ)和超额终身癌症风险(ELCR)评估PM2.5对健康的影响。所研究金属的HQ和ELCR值均在安全范围内。HQ值的大小顺序为Pb >;Cr祝辞而ELCR值的变化趋势为Cr >;Pb祝辞所有年龄组都是Ni。这些发现提供了有关PM2.5浓度和成分、PM2.5潜在来源和健康影响的可靠信息,从而有助于在印度尼西亚雪邦建立空气污染预警系统。
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来源期刊
ACS Earth and Space Chemistry
ACS Earth and Space Chemistry Earth and Planetary Sciences-Geochemistry and Petrology
CiteScore
5.30
自引率
11.80%
发文量
249
期刊介绍: The scope of ACS Earth and Space Chemistry includes the application of analytical, experimental and theoretical chemistry to investigate research questions relevant to the Earth and Space. The journal encompasses the highly interdisciplinary nature of research in this area, while emphasizing chemistry and chemical research tools as the unifying theme. The journal publishes broadly in the domains of high- and low-temperature geochemistry, atmospheric chemistry, marine chemistry, planetary chemistry, astrochemistry, and analytical geochemistry. ACS Earth and Space Chemistry publishes Articles, Letters, Reviews, and Features to provide flexible formats to readily communicate all aspects of research in these fields.
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