Enhancement of Terahertz Radiation from a Transversely Asymmetric Femtosecond Laser Filament

IF 6.7 1区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Jiayu Zhao*, Jiajun Yang, Xiaofeng Li, Feifan Zhu, Li Lao, Yan Peng* and Yiming Zhu*, 
{"title":"Enhancement of Terahertz Radiation from a Transversely Asymmetric Femtosecond Laser Filament","authors":"Jiayu Zhao*,&nbsp;Jiajun Yang,&nbsp;Xiaofeng Li,&nbsp;Feifan Zhu,&nbsp;Li Lao,&nbsp;Yan Peng* and Yiming Zhu*,&nbsp;","doi":"10.1021/acsphotonics.4c0246410.1021/acsphotonics.4c02464","DOIUrl":null,"url":null,"abstract":"<p >Plasma filaments via femtosecond laser ionization in air have been extensively studied as a significant terahertz (THz) source, based on which one particular objective is to enhance the efficiency and intensity of THz radiation. To this end, various strategies have been explored, including modulating the pump laser through temporal asymmetry of the carrier or envelope, or by tailoring the spectral amplitude profile asymmetrically. Apart from the above “asymmetric” operations in time and frequency domains, here we proposed a straightforward and practical method based on the spatial asymmetry. Specifically, an opaque blade was employed to partially obstruct the cross-section of the pump laser beam, resulting in a notable THz power enhancement of up to 60%. To interpret this improvement, we introduced a spatially asymmetric photocurrent mechanism: the created steep gradient of the inhomogeneous laser field enhances the electron drift motion, which in turn generates a stronger transverse current, leading to the observed increase in THz signal strength. To summarize, the proposed experimental method is highly accessible without requiring additional modulation devices, significantly lowering the application threshold. And its mechanism is also versatile, not only enhancing THz transverse wave radiation in both single- and dual-color field configurations, but also potentially applying to other setups, such as tilting focusing lenses or frequency-doubling crystals, warranting a reevaluation of previous studies. Additionally, our approach optimizes energy usage, enabling stronger THz radiation under low-power laser pump conditions and further allowing the blocked laser energy to be redirected for enhanced functionalities.</p>","PeriodicalId":23,"journal":{"name":"ACS Photonics","volume":"12 4","pages":"2034–2043 2034–2043"},"PeriodicalIF":6.7000,"publicationDate":"2025-04-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Photonics","FirstCategoryId":"101","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsphotonics.4c02464","RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

Abstract

Plasma filaments via femtosecond laser ionization in air have been extensively studied as a significant terahertz (THz) source, based on which one particular objective is to enhance the efficiency and intensity of THz radiation. To this end, various strategies have been explored, including modulating the pump laser through temporal asymmetry of the carrier or envelope, or by tailoring the spectral amplitude profile asymmetrically. Apart from the above “asymmetric” operations in time and frequency domains, here we proposed a straightforward and practical method based on the spatial asymmetry. Specifically, an opaque blade was employed to partially obstruct the cross-section of the pump laser beam, resulting in a notable THz power enhancement of up to 60%. To interpret this improvement, we introduced a spatially asymmetric photocurrent mechanism: the created steep gradient of the inhomogeneous laser field enhances the electron drift motion, which in turn generates a stronger transverse current, leading to the observed increase in THz signal strength. To summarize, the proposed experimental method is highly accessible without requiring additional modulation devices, significantly lowering the application threshold. And its mechanism is also versatile, not only enhancing THz transverse wave radiation in both single- and dual-color field configurations, but also potentially applying to other setups, such as tilting focusing lenses or frequency-doubling crystals, warranting a reevaluation of previous studies. Additionally, our approach optimizes energy usage, enabling stronger THz radiation under low-power laser pump conditions and further allowing the blocked laser energy to be redirected for enhanced functionalities.

Abstract Image

横向不对称飞秒激光灯丝对太赫兹辐射的增强
通过飞秒激光电离空气中的等离子体细丝作为一个重要的太赫兹(THz)源已经被广泛研究,在此基础上一个特定的目标是提高太赫兹辐射的效率和强度。为此,已经探索了各种策略,包括通过载流子或包络的时间不对称来调制泵浦激光,或者通过不对称地剪裁光谱幅度轮廓。除了上述时域和频域的“不对称”操作外,本文提出了一种基于空间不对称的简单实用的方法。具体来说,采用不透明叶片来部分阻挡泵浦激光束的横截面,从而显著提高了高达60%的太赫兹功率。为了解释这一改进,我们引入了一种空间不对称的光电流机制:不均匀激光场产生的陡峭梯度增强了电子漂移运动,从而产生更强的横向电流,导致观察到的太赫兹信号强度增加。综上所述,所提出的实验方法不需要额外的调制器件,具有很高的可访问性,显著降低了应用阈值。它的机制也是通用的,不仅在单色和双色场配置中增强太赫兹横波辐射,而且还可能应用于其他设置,例如倾斜聚焦透镜或倍频晶体,这需要对先前的研究进行重新评估。此外,我们的方法优化了能量使用,在低功率激光泵浦条件下实现更强的太赫兹辐射,并进一步允许被阻挡的激光能量重新定向以增强功能。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 求助全文
来源期刊
ACS Photonics
ACS Photonics NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
11.90
自引率
5.70%
发文量
438
审稿时长
2.3 months
期刊介绍: Published as soon as accepted and summarized in monthly issues, ACS Photonics will publish Research Articles, Letters, Perspectives, and Reviews, to encompass the full scope of published research in this field.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:604180095
Book学术官方微信