{"title":"Breakup dynamics of viscous bubbles in heart-shaped microchannel: Mechanisms and predictive models","authors":"Jiahua Hu, Wei Zhang, Xin Xu, Feiyu Gao, Yaqi Hou","doi":"10.1016/j.ces.2025.121666","DOIUrl":null,"url":null,"abstract":"To enhance the gas–liquid mass transfer efficiency in high-viscosity fluids within heart-shaped microchannels, this study systematically investigated the bubble breakup dynamics at the arc-shaped junction of heart-shaped microchannel under different viscosities of glycerol solution. High-speed camera observed that bubble breakup at the arc-shaped junction could be divided into three cases: breakup with obstruction, breakup with tunnel, and squeezing breakup. The occurrence of bubble breakup is related to the bubble equivalent length (<em>l</em><sub>0</sub>/<em>w</em><sub>0</sub>) and the capillary number (<em>Ca</em>), and the bubble breakup pattern transition rule under different liquid phase viscosities was obtained through data analysis. Furthermore, the effects of the bubble equivalent length, total capillary number, liquid phase viscosity (<em>μ</em><sub>L</sub>), and velocity of the rear-bubble (<em>U</em><sub>g</sub>) on bubble squeezing breakup were investigated. The data analysis showed that <em>U</em><sub>g</sub> significantly affected the power-law indices <em>α</em> and <em>β</em>, increasing <em>α</em> by 23.8 % and <em>β</em> by 43.9 %, respectively. In addition, this study proposed a three-dimensional surface model <em>l</em><sub>0</sub>/<em>w</em><sub>0</sub> = <em>a</em>(<em>U</em><sub>g</sub>/<em>U</em><sub>in</sub>)<em><sup>b</sup>Ca<sup>c</sup></em> for the first time to predict whether bubble squeezing breakup occurs, offering a robust theoretical framework for controlling bubble breakup in high-viscosity systems. This study deepens the understanding of bubble breakup dynamics in high-viscosity systems and provides a theoretical foundation for structural optimization of heart-shaped microchannels.","PeriodicalId":271,"journal":{"name":"Chemical Engineering Science","volume":"90 1","pages":""},"PeriodicalIF":4.1000,"publicationDate":"2025-04-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Chemical Engineering Science","FirstCategoryId":"5","ListUrlMain":"https://doi.org/10.1016/j.ces.2025.121666","RegionNum":2,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
引用次数: 0
Abstract
To enhance the gas–liquid mass transfer efficiency in high-viscosity fluids within heart-shaped microchannels, this study systematically investigated the bubble breakup dynamics at the arc-shaped junction of heart-shaped microchannel under different viscosities of glycerol solution. High-speed camera observed that bubble breakup at the arc-shaped junction could be divided into three cases: breakup with obstruction, breakup with tunnel, and squeezing breakup. The occurrence of bubble breakup is related to the bubble equivalent length (l0/w0) and the capillary number (Ca), and the bubble breakup pattern transition rule under different liquid phase viscosities was obtained through data analysis. Furthermore, the effects of the bubble equivalent length, total capillary number, liquid phase viscosity (μL), and velocity of the rear-bubble (Ug) on bubble squeezing breakup were investigated. The data analysis showed that Ug significantly affected the power-law indices α and β, increasing α by 23.8 % and β by 43.9 %, respectively. In addition, this study proposed a three-dimensional surface model l0/w0 = a(Ug/Uin)bCac for the first time to predict whether bubble squeezing breakup occurs, offering a robust theoretical framework for controlling bubble breakup in high-viscosity systems. This study deepens the understanding of bubble breakup dynamics in high-viscosity systems and provides a theoretical foundation for structural optimization of heart-shaped microchannels.
期刊介绍:
Chemical engineering enables the transformation of natural resources and energy into useful products for society. It draws on and applies natural sciences, mathematics and economics, and has developed fundamental engineering science that underpins the discipline.
Chemical Engineering Science (CES) has been publishing papers on the fundamentals of chemical engineering since 1951. CES is the platform where the most significant advances in the discipline have ever since been published. Chemical Engineering Science has accompanied and sustained chemical engineering through its development into the vibrant and broad scientific discipline it is today.