{"title":"Full Electrical Manipulation of Perpendicular Magnetization in [111]-Orientated Pt/Co Heterostructure Enabled by Anisotropic Epitaxial Strain","authors":"Haiming Xu, Qirui Cui, Jijun Yun, Yunchi Zhao, Congli He, Xiaowei Lv, Tengyu Guo, Zengtai Zhu, Lili Luo, Hao Wu, Shouguo Wang, Renchao Che, Yalu Zuo, Guoqiang Yu, Hongxin Yang, Li Xi, Baoshan Cui","doi":"10.1021/acs.nanolett.5c00699","DOIUrl":null,"url":null,"abstract":"The effective manipulation of perpendicular magnetization through spin–orbit torque (SOT) holds great promise for magnetic memory and spin-logic device. However, field-free SOT switching of perpendicular magnetization remains a challenge for conventional materials with high symmetry. This study elucidates a full electrical manipulation of the perpendicular magnetization in an epitaxial [111]-orientated Pt/Co heterostructure. A large anisotropic epitaxial strain induces a symmetry transition from the ideal <i>C</i><sub>3<i>v</i></sub> to <i>C</i><sub>1<i>v</i></sub>, attributed to the mismatch between [11<span>2</span>] and [1<span>1</span>0] directions. The anisotropic strain also generates a noteworthy in-plane magnetization component along the [11<span>2</span>] direction, further breaking magnetic symmetry. Notably, the high-temperature performance under 393 K highlights the robustness of strain-induced in-plane symmetry breaking. Furthermore, eight Boolean logic operations have been demonstrated within a single SOT device. This research presents a method for harnessing epitaxial strain to break in-plane symmetry, which may open a new avenue in practical SOT devices.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"108 1","pages":""},"PeriodicalIF":9.6000,"publicationDate":"2025-04-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Letters","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acs.nanolett.5c00699","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
The effective manipulation of perpendicular magnetization through spin–orbit torque (SOT) holds great promise for magnetic memory and spin-logic device. However, field-free SOT switching of perpendicular magnetization remains a challenge for conventional materials with high symmetry. This study elucidates a full electrical manipulation of the perpendicular magnetization in an epitaxial [111]-orientated Pt/Co heterostructure. A large anisotropic epitaxial strain induces a symmetry transition from the ideal C3v to C1v, attributed to the mismatch between [112] and [110] directions. The anisotropic strain also generates a noteworthy in-plane magnetization component along the [112] direction, further breaking magnetic symmetry. Notably, the high-temperature performance under 393 K highlights the robustness of strain-induced in-plane symmetry breaking. Furthermore, eight Boolean logic operations have been demonstrated within a single SOT device. This research presents a method for harnessing epitaxial strain to break in-plane symmetry, which may open a new avenue in practical SOT devices.
期刊介绍:
Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including:
- Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale
- Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies
- Modeling and simulation of synthetic, assembly, and interaction processes
- Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance
- Applications of nanoscale materials in living and environmental systems
Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.