{"title":"A sensitive, robust, high temperature resistant flexible piezoelectric sensor based on SiC/AlN hybrid thin films","authors":"Xing Jia , Zhaohui Weng , Haofeng Qiu , Wei Xue , Ningbo Liao","doi":"10.1016/j.surfin.2025.106419","DOIUrl":null,"url":null,"abstract":"<div><div>Flexible pressure sensors generate significant attention for their promising applications in wearable electronic devices and human-computer interaction systems. Specially, high-temperature resistant flexible sensors are urgently demanded to detect physiological characteristics of human such as firefighters and deep-sea workers in harsh environments. In this study, a highly sensitive, waterproof, high-temperature resistant flexible silicon carbide (SiC)/aluminum nitride (AlN) sensor is proposed, and prepared by magnetron sputtering hybrid piezoelectric thin-film on silica gel substrate. The SiC/AlN thin-film sensor exhibits a high sensitivity of 7.44 mV/kPa and high R<sup>2</sup> value of 0.9159 at a pressure below 150 kPa, together with improved piezoelectric performance of 52.27% compared to that of SiC sensor. In addition, the flexible piezoelectric sensor can practically recognize human motions of sitting to standing, walking and running and shows excellent reliability upon 4000 cycling loading. The SiC/AlN sensor also exhibits high sensitivity of 3.358 mV/kPa at high temperatures and presents excellent stability up to 170°C. First-principles calculations suggest that the incorporation of AlN significantly reduces band gap of SiC, with enhanced charge transport and improved carrier transport efficiency. This work provides an experimental and numerical perspective for designing high performance, low-cost flexible sensors for harsh environments.</div></div>","PeriodicalId":22081,"journal":{"name":"Surfaces and Interfaces","volume":"64 ","pages":"Article 106419"},"PeriodicalIF":5.7000,"publicationDate":"2025-04-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Surfaces and Interfaces","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2468023025006765","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
引用次数: 0
Abstract
Flexible pressure sensors generate significant attention for their promising applications in wearable electronic devices and human-computer interaction systems. Specially, high-temperature resistant flexible sensors are urgently demanded to detect physiological characteristics of human such as firefighters and deep-sea workers in harsh environments. In this study, a highly sensitive, waterproof, high-temperature resistant flexible silicon carbide (SiC)/aluminum nitride (AlN) sensor is proposed, and prepared by magnetron sputtering hybrid piezoelectric thin-film on silica gel substrate. The SiC/AlN thin-film sensor exhibits a high sensitivity of 7.44 mV/kPa and high R2 value of 0.9159 at a pressure below 150 kPa, together with improved piezoelectric performance of 52.27% compared to that of SiC sensor. In addition, the flexible piezoelectric sensor can practically recognize human motions of sitting to standing, walking and running and shows excellent reliability upon 4000 cycling loading. The SiC/AlN sensor also exhibits high sensitivity of 3.358 mV/kPa at high temperatures and presents excellent stability up to 170°C. First-principles calculations suggest that the incorporation of AlN significantly reduces band gap of SiC, with enhanced charge transport and improved carrier transport efficiency. This work provides an experimental and numerical perspective for designing high performance, low-cost flexible sensors for harsh environments.
期刊介绍:
The aim of the journal is to provide a respectful outlet for ''sound science'' papers in all research areas on surfaces and interfaces. We define sound science papers as papers that describe new and well-executed research, but that do not necessarily provide brand new insights or are merely a description of research results.
Surfaces and Interfaces publishes research papers in all fields of surface science which may not always find the right home on first submission to our Elsevier sister journals (Applied Surface, Surface and Coatings Technology, Thin Solid Films)