High-Performance Zero-Powered InHfO/GaN Photodetectors for Ultraviolet Image Sensing Systems

IF 4.3 3区 材料科学 Q1 ENGINEERING, ELECTRICAL & ELECTRONIC
Bojia Chen, Jiyuan Zhu, Shice Wei, Yu Zhang, Xuefeng Wu*, David Wei Zhang, Qing-Qing Sun, Li Ji* and Shen Hu*, 
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Abstract

The advancement of photodetector technology, particularly in enhancing response speed and photosensitivity, is crucial for the development of high-density optical arrays and image sensing systems. Wide-bandgap indium oxide with high electron mobility is ideal for fabricating ultraviolet photodetectors capable of high-speed response. Nonetheless, photodetectors based on single indium oxide semiconductors exhibit a large dark current and high energy consumption, which hinders their practical application in photodetection. In this research, we fabricated an indium–hafnium oxide/gallium nitride (IHO/GaN) ultraviolet photodetector via atomic layer deposition. This method not only reduces the photodetector’s response time but also allows it to realize optoelectronic conversion without external power. Simultaneously, the optimized photodetector exhibits remarkable performance metrics under 280 nm ultraviolet illumination, including a responsivity of 375 mA/W, a detectivity of 4.4 × 1012 Jones, a photo-dark current ratio of 3.3 × 105 %, and a rise/fall time of 42/66 ms. The exceptional performance is credited to the swift separation of photogenerated electron–hole pairs, facilitated by the substantial built-in electric field present in the depletion region at the p–n junction interface. Additionally, arrayed IHO/GaN photodetectors demonstrate potential to apply in image recognition systems, providing an effective strategy for constructing high-performance zero-powered ultraviolet detectors for optical imaging.

Abstract Image

用于紫外图像传感系统的高性能零功率InHfO/GaN光电探测器
光电探测器技术的进步,特别是在提高响应速度和光敏性方面的进步,对高密度光学阵列和图像传感系统的发展至关重要。具有高电子迁移率的宽禁带氧化铟是制造高速响应紫外光电探测器的理想材料。然而,基于单氧化铟半导体的光电探测器具有较大的暗电流和高能量消耗,这阻碍了它们在光电探测中的实际应用。本研究采用原子层沉积法制备了氧化铟铪/氮化镓(IHO/GaN)紫外光电探测器。这种方法不仅缩短了光电探测器的响应时间,而且使其可以在没有外部电源的情况下实现光电转换。同时,优化后的光电探测器在280 nm紫外光照射下表现出了显著的性能指标,包括响应度为375 mA/W,探测率为4.4 × 1012 Jones,光暗电流比为3.3 × 105%,上升/下降时间为42/66 ms。这种优异的性能归功于光生电子-空穴对的快速分离,这是由p-n结界面耗尽区存在的大量内置电场促进的。此外,阵列IHO/GaN光电探测器显示出应用于图像识别系统的潜力,为构建用于光学成像的高性能零功率紫外探测器提供了有效的策略。
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来源期刊
CiteScore
7.20
自引率
4.30%
发文量
567
期刊介绍: ACS Applied Electronic Materials is an interdisciplinary journal publishing original research covering all aspects of electronic materials. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials science, engineering, optics, physics, and chemistry into important applications of electronic materials. Sample research topics that span the journal's scope are inorganic, organic, ionic and polymeric materials with properties that include conducting, semiconducting, superconducting, insulating, dielectric, magnetic, optoelectronic, piezoelectric, ferroelectric and thermoelectric. Indexed/​Abstracted: Web of Science SCIE Scopus CAS INSPEC Portico
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