Bojia Chen, Jiyuan Zhu, Shice Wei, Yu Zhang, Xuefeng Wu*, David Wei Zhang, Qing-Qing Sun, Li Ji* and Shen Hu*,
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引用次数: 0
Abstract
The advancement of photodetector technology, particularly in enhancing response speed and photosensitivity, is crucial for the development of high-density optical arrays and image sensing systems. Wide-bandgap indium oxide with high electron mobility is ideal for fabricating ultraviolet photodetectors capable of high-speed response. Nonetheless, photodetectors based on single indium oxide semiconductors exhibit a large dark current and high energy consumption, which hinders their practical application in photodetection. In this research, we fabricated an indium–hafnium oxide/gallium nitride (IHO/GaN) ultraviolet photodetector via atomic layer deposition. This method not only reduces the photodetector’s response time but also allows it to realize optoelectronic conversion without external power. Simultaneously, the optimized photodetector exhibits remarkable performance metrics under 280 nm ultraviolet illumination, including a responsivity of 375 mA/W, a detectivity of 4.4 × 1012 Jones, a photo-dark current ratio of 3.3 × 105 %, and a rise/fall time of 42/66 ms. The exceptional performance is credited to the swift separation of photogenerated electron–hole pairs, facilitated by the substantial built-in electric field present in the depletion region at the p–n junction interface. Additionally, arrayed IHO/GaN photodetectors demonstrate potential to apply in image recognition systems, providing an effective strategy for constructing high-performance zero-powered ultraviolet detectors for optical imaging.
期刊介绍:
ACS Applied Electronic Materials is an interdisciplinary journal publishing original research covering all aspects of electronic materials. The journal is devoted to reports of new and original experimental and theoretical research of an applied nature that integrate knowledge in the areas of materials science, engineering, optics, physics, and chemistry into important applications of electronic materials. Sample research topics that span the journal's scope are inorganic, organic, ionic and polymeric materials with properties that include conducting, semiconducting, superconducting, insulating, dielectric, magnetic, optoelectronic, piezoelectric, ferroelectric and thermoelectric.
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