Quantum Emitters in Flux Grown hBN

IF 3.2 2区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
Evan Williams, Angus Gale*, Jake Horder, Dominic Scognamiglio, Milos Toth and Igor Aharonovich, 
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引用次数: 0

Abstract

Hexagonal boron nitride (hBN) is an emerging material for use in quantum technologies, hosting bright and stable single photon emitters (SPEs). The B-center is one promising SPE in hBN, due to the near-deterministic creation methods and regular emission wavelength. However, incorporation of B-centers in high-quality crystals remains challenging, typically relying on additional postgrowth methods to increase creation efficiency. Here, we have demonstrated controlled carbon doping of hBN during growth, using a metal flux-based method to increase the efficiency of B-center creation. Importantly, single B-centers with g(2)(0) < 0.5 were able to be generated in the as-grown hBN when carbon additions during growth exceeded 2.5 wt % C. Resonant excitation measurements revealed line widths of 3.5 GHz with only moderate spectral diffusion present, demonstrating the applicability of the as-grown hBN as a host for high-quality B-centers.

Abstract Image

通量生长hBN中的量子发射体
六方氮化硼(hBN)是一种用于量子技术的新兴材料,承载明亮和稳定的单光子发射器(spe)。由于b中心的形成方法接近确定,且发射波长规则,是一种很有前途的hBN固相萃取。然而,在高质量晶体中加入b中心仍然具有挑战性,通常依赖于额外的生长后方法来提高创造效率。在这里,我们展示了在生长过程中控制碳掺杂的hBN,使用基于金属助熔剂的方法来提高b中心生成的效率。重要的是,单b中心具有g(2)(0) <;当生长过程中的碳添加量超过2.5 wt % c时,在生长的hBN中能够产生0.5。共振激发测量显示线宽为3.5 GHz,仅存在中等的光谱扩散,表明生长的hBN作为高质量b中心的宿主的适用性。
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来源期刊
Crystal Growth & Design
Crystal Growth & Design 化学-材料科学:综合
CiteScore
6.30
自引率
10.50%
发文量
650
审稿时长
1.9 months
期刊介绍: The aim of Crystal Growth & Design is to stimulate crossfertilization of knowledge among scientists and engineers working in the fields of crystal growth, crystal engineering, and the industrial application of crystalline materials. Crystal Growth & Design publishes theoretical and experimental studies of the physical, chemical, and biological phenomena and processes related to the design, growth, and application of crystalline materials. Synergistic approaches originating from different disciplines and technologies and integrating the fields of crystal growth, crystal engineering, intermolecular interactions, and industrial application are encouraged.
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