Directional Light Scattering of a Single Si Nanoparticle Revealed by Three-Dimensional Near-Field Optical Microscopy

IF 4.6 2区 化学 Q2 CHEMISTRY, PHYSICAL
Kohei Imura, Takuya Matsuura
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引用次数: 0

Abstract

Manipulation of light propagation is indispensable for the development of photonic circuits and nano-optical devices. In this study, we investigated the optical properties of Mie resonances in a single Si nanoparticle via dark field and near-field optical microscopy. The dark field spectrum of the nanoparticle exhibits electric and magnetic dipolar modes in the visible to near-infrared spectral region. The near-field spectrum shows red-shifted and enhanced peaks due to these resonances. From the electromagnetic simulation, we revealed that these unique near-field characteristics originate from the constructive interaction of the incident and scattered fields. We also performed three-dimensional near-field microscopy and demonstrated that the magnetic dipolar mode results in wider spatial extension and directional forward scattering than does the electric dipolar mode does. These findings indicate that the interaction of the magnetic dipolar mode with near-field light is desirable for controlling light propagation in various applications.

Abstract Image

三维近场光学显微镜研究单硅纳米颗粒的定向光散射
光的传播控制对于光子电路和纳米光学器件的发展是必不可少的。在这项研究中,我们通过暗场和近场光学显微镜研究了单个Si纳米颗粒中的Mie共振的光学性质。纳米粒子的暗场光谱在可见光至近红外光谱区表现为电偶极模式和磁偶极模式。由于这些共振,近场光谱显示出红移和增强的峰。通过电磁模拟,我们发现这些独特的近场特性源于入射场和散射场的建设性相互作用。我们还进行了三维近场显微镜,并证明磁偶极子模式比电偶极子模式产生更宽的空间延伸和定向前向散射。这些发现表明,磁偶极子模式与近场光的相互作用是在各种应用中控制光传播所需要的。
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来源期刊
The Journal of Physical Chemistry Letters
The Journal of Physical Chemistry Letters CHEMISTRY, PHYSICAL-NANOSCIENCE & NANOTECHNOLOGY
CiteScore
9.60
自引率
7.00%
发文量
1519
审稿时长
1.6 months
期刊介绍: The Journal of Physical Chemistry (JPC) Letters is devoted to reporting new and original experimental and theoretical basic research of interest to physical chemists, biophysical chemists, chemical physicists, physicists, material scientists, and engineers. An important criterion for acceptance is that the paper reports a significant scientific advance and/or physical insight such that rapid publication is essential. Two issues of JPC Letters are published each month.
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