Reconfigurable Terahertz Metamaterials Based on the Refractive Index Change of Epitaxial Vanadium Dioxide Films Across the Metal-Insulator Transition.

Abstract

The intrinsic metal-insulator transition (MIT) of VO₂ films near room temperature presents significant potential for reconfigurable metamaterials in the terahertz (THz) frequency range. While previous designs primarily focused on changes in electrical conductivity across the MIT, the accompanying dielectric changes due to the mesoscopic carrier confinement effect have been largely unexplored. In this study, we integrate asymmetric split-ring resonators on 35 nm epitaxial VO₂ film and identify a "dielectric window" at the early stages of the MIT. This is characterized by a redshift in the resonant frequency without a significant degradation in the resonant quality. This phenomenon is attributed to an inhomogeneous phase transition in the VO₂ film, which induces a purely dielectric change at the onset of the MIT, while the electrical conductivity transition occurs later, slightly above the percolation threshold. Our findings provide deeper insights into the THz properties of VO₂ films and pave the way for dielectric-based, VO₂ hybrid reconfigurable metamaterials.