Using AOD and UVAI to Reduce the Uncertainties in Wildfire Emission and Air Quality Modeling

IF 3.8 2区 地球科学 Q2 METEOROLOGY & ATMOSPHERIC SCIENCES
Yunyao Li, Daniel Tong, Yeseul Jeon, Benjamin Seiyon Lee, Jaewoo Park, Shobha Kondragunta, Xiaoyang Zhang, Naphat Siripun, Stephanie Song, Charu Mehta, Jenny Zhao Chen
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Abstract

Wildfires are a major natural source of atmospheric aerosols, leading to air quality degradation and adverse human health effects. Accurate prediction of air quality effects from wildfires remains challenging due to uncertainties in fire emission estimates. To enhance the accuracy of fire emissions used in air quality forecast models, we developed a method that utilizes satellite aerosol optical depth (AOD) observations and air quality simulations to calculate dynamic emission scaling factors and improve wildfire air quality forecasts. TROPOMI (TROPOspheric Monitoring Instrument) UV Aerosol Index (UVAI) data are employed to fill AOD gaps under thick smoke using two approaches: a regression model and an artificial intelligence model. The scaling factor method was applied to NOAA blended Global Biomass Burning Emissions Product. The emission scaling factors exhibited significant variability across different fire points, highlighting the need for point-specific scaling factors. On average, scaling factors were less than 1.0 (indicating emission overestimation) during the initial stages of fire events but exceeded 1.0 (suggesting underestimation) after 7 days of fire duration. An inverse relationship between scaling factors and fire radiative power (FRP) was observed, with emission underestimation for low-intensity fires (FRP <5 MW) and substantial overestimation for high-intensity fires (FRP >500 MW). The improved fire emissions were employed in the air quality model for the 2020 US Gigafire event. Utilizing emission scaling factors reduced model bias, increased the correlation and hit rate of PM2.5 exceedance prediction, demonstrating the potential of using emission scaling factors for improving air quality forecasting during wildfire events.

Abstract Image

野火是大气气溶胶的主要自然来源,会导致空气质量下降并对人类健康造成不利影响。由于火灾排放量估算的不确定性,准确预测野火对空气质量的影响仍然具有挑战性。为了提高空气质量预测模型中使用的火灾排放量的准确性,我们开发了一种方法,利用卫星气溶胶光学深度(AOD)观测和空气质量模拟来计算动态排放缩放因子,从而改善野火空气质量预测。利用 TROPOMI(TROPOspheric Monitoring Instrument)紫外线气溶胶指数(UVAI)数据,采用回归模型和人工智能模型两种方法填补浓烟下的 AOD 缺口。缩放因子法适用于 NOAA 混合全球生物质燃烧排放产品。排放缩放因子在不同火点之间表现出显著的差异性,突出表明需要特定火点的缩放因子。平均而言,在火灾事件的初始阶段,缩放因子小于 1.0(表明高估了排放量),但在火灾持续 7 天后,缩放因子超过了 1.0(表明低估了排放量)。缩放因子与火灾辐射功率(FRP)之间存在反比关系,低强度火灾(FRP <5 MW)的排放量被低估,而高强度火灾(FRP >500 MW)的排放量被大幅高估。改进后的火灾排放被用于 2020 年美国 Gigafire 事件的空气质量模型。使用排放缩放因子减少了模型偏差,提高了 PM2.5 超标预测的相关性和命中率,证明了使用排放缩放因子改进野火事件期间空气质量预测的潜力。
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来源期刊
Journal of Geophysical Research: Atmospheres
Journal of Geophysical Research: Atmospheres Earth and Planetary Sciences-Geophysics
CiteScore
7.30
自引率
11.40%
发文量
684
期刊介绍: JGR: Atmospheres publishes articles that advance and improve understanding of atmospheric properties and processes, including the interaction of the atmosphere with other components of the Earth system.
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