{"title":"Multi-Factor Multi-Level Optimization of MOFs-derivatives for Promoting Catalyst fabrication.","authors":"Ruirui Yun, Peiwei Zhao, Yuqing Zhang, Lele Gao, Yu Wang, Yimin Sun, Shizhong Luo","doi":"10.1002/cplu.202500110","DOIUrl":null,"url":null,"abstract":"<p><p>To design catalysts with high performance on the heterogeneous catalysis fields has puzzled many scientists due to the multifarious repeated experiments which takes most of their time. Herein, a multi-factor and multi-level experimental design (M2ED) with an artificial neural network (ANN) has been performed to optimize the catalyst synthesis tactic. During the process, 5 factors within one experiment was considered to establish a neural network model to pick out the optimal synthesis condition. Excitingly, the as-synthesized catalyst according to the above strategy displays superior catalytic activity to the other similar synthesis tactics. This work not only fabricates a catalyst with extremely catalytic performance but also provides new insights into constructing catalysts with special function efficiently.</p>","PeriodicalId":148,"journal":{"name":"ChemPlusChem","volume":" ","pages":"e202500110"},"PeriodicalIF":3.0000,"publicationDate":"2025-03-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ChemPlusChem","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1002/cplu.202500110","RegionNum":4,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
To design catalysts with high performance on the heterogeneous catalysis fields has puzzled many scientists due to the multifarious repeated experiments which takes most of their time. Herein, a multi-factor and multi-level experimental design (M2ED) with an artificial neural network (ANN) has been performed to optimize the catalyst synthesis tactic. During the process, 5 factors within one experiment was considered to establish a neural network model to pick out the optimal synthesis condition. Excitingly, the as-synthesized catalyst according to the above strategy displays superior catalytic activity to the other similar synthesis tactics. This work not only fabricates a catalyst with extremely catalytic performance but also provides new insights into constructing catalysts with special function efficiently.
期刊介绍:
ChemPlusChem is a peer-reviewed, general chemistry journal that brings readers the very best in multidisciplinary research centering on chemistry. It is published on behalf of Chemistry Europe, an association of 16 European chemical societies.
Fully comprehensive in its scope, ChemPlusChem publishes articles covering new results from at least two different aspects (subfields) of chemistry or one of chemistry and one of another scientific discipline (one chemistry topic plus another one, hence the title ChemPlusChem). All suitable submissions undergo balanced peer review by experts in the field to ensure the highest quality, originality, relevance, significance, and validity.