Matthew Yeung, Lu-Ting Chou, Felix Ritzkowsky, Marco Turchetti, Karl K. Berggren, Shih-Hsuan Chia, Phillip D. Keathley
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引用次数: 0
Abstract
Lightwave electronics offer transformative field-level precision and control at high optical frequencies. While recent advances show that lightwave-driven electron emission from nanoantennas enables time-domain, field-resolved analysis of optical waveforms through a small-signal analysis, the effect of the gate waveform on the measurement transfer function remains unexplored. By generating electrons with a 10-cycle pulse in the optical tunneling regime and perturbing the response with a 1.5-cycle pulse, we experimentally measure the bandwidth limitations imposed by the electron emission process. By comparing these measurements with TDSE simulations and analytical models, we reveal the temporal properties of the electronic response and its impact on the small-signal transfer function. Our results test and confirm the accuracy of the Fowler–Nordheim model in estimating the lightwave electronic response from noble metals. We envision extending these techniques to multi-octave-spanning signals for precise characterization of sub-cycle electronic responses through harmonic frequency mixing.
期刊介绍:
Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including:
- Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale
- Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies
- Modeling and simulation of synthetic, assembly, and interaction processes
- Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance
- Applications of nanoscale materials in living and environmental systems
Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.