Chenhao Zeng , Hongjian Lin , WanChang Lai , Guangxi Wang , Ningbo Liu , Zhongshan Duan , Youjun Wang , He Sun , Bing Qin , Xiaojie Feng , Yuanye Lin , Haoyuan Lu
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引用次数: 0
Abstract
In environmental gamma radioactivity measurements, the measurement of potassium, uranium, and thorium is crucial for strategic resource exploration, geological surveys, and environmental background investigations. This study focused on CeBr3 detector measurements and discovered that artificial radionuclides affected the intrinsic peaks and peak positions in the regions of interest for potassium, uranium, and thorium, resulting in offsets and distortions in the energy spectrum. Based on principal component analysis and linear regression, the study corrected the interference of artificial radionuclides in the measurements of potassium, uranium, and thorium. The results demonstrated that the peak offset was effectively corrected, with a maximum offset of 0.8 channels, compared to a maximum offset of 6.5 channels before correction. Additionally, correcting the peak area changes yielded better results, effectively reducing the errors in peak area calculations. Specifically, the error in peak area calculations was reduced from 10.52 % to 1.62 % for potassium, from 13.48 % to 1.79 % for uranium, and from 7.00 % to 4.96 % for thorium. The study successfully mitigated the peak position shifts and peak area variations caused by the counting contributions of artificial radionuclide 137Cs to the regions of interest for potassium, uranium, and thorium, thereby improving the accuracy of peak area calculations. The analytical method effectively addresses the issue of gamma energy spectrum offset and deformation, holding significant research significance and practical value in various applications, including aerial gamma energy spectrum measurements, environmental radioactivity measurements, geological exploration, and mineral investigations.
期刊介绍:
Radiation Physics and Chemistry is a multidisciplinary journal that provides a medium for publication of substantial and original papers, reviews, and short communications which focus on research and developments involving ionizing radiation in radiation physics, radiation chemistry and radiation processing.
The journal aims to publish papers with significance to an international audience, containing substantial novelty and scientific impact. The Editors reserve the rights to reject, with or without external review, papers that do not meet these criteria. This could include papers that are very similar to previous publications, only with changed target substrates, employed materials, analyzed sites and experimental methods, report results without presenting new insights and/or hypothesis testing, or do not focus on the radiation effects.