Lanyue Zhang, Zhanhong Yuan, Xiaotong Fu, Shiang Shi, Xiang Chen, Pan Chen, Dongdong Ye
{"title":"Biomass-Derived Gradient and Aligned Structured Aerogel for Sustainable Agricultural Irrigation","authors":"Lanyue Zhang, Zhanhong Yuan, Xiaotong Fu, Shiang Shi, Xiang Chen, Pan Chen, Dongdong Ye","doi":"10.1021/acs.nanolett.5c00520","DOIUrl":null,"url":null,"abstract":"Interface evaporation-driven hydroelectric systems integrating water purification and energy collection offer the potential for sustainable agricultural irrigation. However, achieving high evaporation rates and efficient energy harvesting poses challenges, particularly in optimizing evaporation and water transport. This study develops a gradient-aligned structured aerogel (GA aerogel), composed of biomass materials such as cellulose and chitosan, which utilizes efficient water transport through aligned cellulose channels, unique ion management in nanoscale channels, and chitosan’s ability to reduce evaporation energy consumption, thereby enhancing water and energy harvesting performance. The GA aerogel achieves a solar absorption rate of 91.4%, an evaporation rate of 2.5 kg m<sup>–2</sup> h<sup>–1</sup>, an output power of 680 nW cm<sup>–2</sup>, and stable operation for over 120 h. Furthermore, by integrating a series array with capacitive energy storage, the system utilizes harvested electrical energy to irrigate plants with purified water, promoting sustainable agriculture and providing insights for designing biomass-based solar evaporators.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"23 1","pages":""},"PeriodicalIF":9.6000,"publicationDate":"2025-03-23","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Letters","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acs.nanolett.5c00520","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Interface evaporation-driven hydroelectric systems integrating water purification and energy collection offer the potential for sustainable agricultural irrigation. However, achieving high evaporation rates and efficient energy harvesting poses challenges, particularly in optimizing evaporation and water transport. This study develops a gradient-aligned structured aerogel (GA aerogel), composed of biomass materials such as cellulose and chitosan, which utilizes efficient water transport through aligned cellulose channels, unique ion management in nanoscale channels, and chitosan’s ability to reduce evaporation energy consumption, thereby enhancing water and energy harvesting performance. The GA aerogel achieves a solar absorption rate of 91.4%, an evaporation rate of 2.5 kg m–2 h–1, an output power of 680 nW cm–2, and stable operation for over 120 h. Furthermore, by integrating a series array with capacitive energy storage, the system utilizes harvested electrical energy to irrigate plants with purified water, promoting sustainable agriculture and providing insights for designing biomass-based solar evaporators.
期刊介绍:
Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including:
- Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale
- Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies
- Modeling and simulation of synthetic, assembly, and interaction processes
- Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance
- Applications of nanoscale materials in living and environmental systems
Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.