Realizing a topological diode effect on the surface of a topological Kondo insulator

IF 9.4 1区 综合性期刊 Q1 MULTIDISCIPLINARY SCIENCES
Jiawen Zhang, Zhenqi Hua, Chengwei Wang, Michael Smidman, David Graf, Sean Thomas, Priscila F. S. Rosa, Steffen Wirth, Xi Dai, Peng Xiong, Huiqiu Yuan, Xiaoyu Wang, Lin Jiao
{"title":"Realizing a topological diode effect on the surface of a topological Kondo insulator","authors":"Jiawen Zhang, Zhenqi Hua, Chengwei Wang, Michael Smidman, David Graf, Sean Thomas, Priscila F. S. Rosa, Steffen Wirth, Xi Dai, Peng Xiong, Huiqiu Yuan, Xiaoyu Wang, Lin Jiao","doi":"10.1073/pnas.2417709122","DOIUrl":null,"url":null,"abstract":"Introducing the concept of topology into material science has sparked a revolution from classic electronic and optoelectronic devices to topological quantum devices. The latter has potential for transferring energy and information with unprecedented efficiency. Here, we demonstrate a topological diode effect on the surface of a three-dimensional material, SmB <jats:inline-formula> <mml:math xmlns:mml=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\" overflow=\"scroll\"> <mml:msub> <mml:mrow/> <mml:mn>6</mml:mn> </mml:msub> </mml:math> </jats:inline-formula> , a candidate topological Kondo insulator. The diode effect is evidenced by pronounced rectification and photogalvanic effects under electromagnetic modulation and radiation at radio frequency. Our experimental results and modeling suggest that these prominent effects are intimately tied to the spatially inhomogeneous formation of topological surface states (TSS) at the intermediate temperature. This work provides a manner of breaking the mirror symmetry (in addition to the inversion symmetry), resulting in the formation of <jats:inline-formula> <mml:math xmlns:mml=\"http://www.w3.org/1998/Math/MathML\" display=\"inline\" overflow=\"scroll\"> <mml:mrow> <mml:mi mathvariant=\"italic\">pn</mml:mi> </mml:mrow> </mml:math> </jats:inline-formula> -junctions between puddles of metallic TSS. This effect paves the way for efficient current rectifiers or energy-harvesting devices working down to radio frequency range at low temperature, which could be extended to high temperatures using other topological insulators with large bulk gap.","PeriodicalId":20548,"journal":{"name":"Proceedings of the National Academy of Sciences of the United States of America","volume":"27 1","pages":""},"PeriodicalIF":9.4000,"publicationDate":"2025-03-20","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Proceedings of the National Academy of Sciences of the United States of America","FirstCategoryId":"103","ListUrlMain":"https://doi.org/10.1073/pnas.2417709122","RegionNum":1,"RegionCategory":"综合性期刊","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MULTIDISCIPLINARY SCIENCES","Score":null,"Total":0}
引用次数: 0

Abstract

Introducing the concept of topology into material science has sparked a revolution from classic electronic and optoelectronic devices to topological quantum devices. The latter has potential for transferring energy and information with unprecedented efficiency. Here, we demonstrate a topological diode effect on the surface of a three-dimensional material, SmB 6 , a candidate topological Kondo insulator. The diode effect is evidenced by pronounced rectification and photogalvanic effects under electromagnetic modulation and radiation at radio frequency. Our experimental results and modeling suggest that these prominent effects are intimately tied to the spatially inhomogeneous formation of topological surface states (TSS) at the intermediate temperature. This work provides a manner of breaking the mirror symmetry (in addition to the inversion symmetry), resulting in the formation of pn -junctions between puddles of metallic TSS. This effect paves the way for efficient current rectifiers or energy-harvesting devices working down to radio frequency range at low temperature, which could be extended to high temperatures using other topological insulators with large bulk gap.
将拓扑学概念引入材料科学引发了一场从传统电子和光电设备到拓扑量子设备的革命。后者有望以前所未有的效率传输能量和信息。在这里,我们展示了三维材料 SmB 6(一种候选拓扑近藤绝缘体)表面的拓扑二极管效应。在射频电磁调制和辐射作用下,二极管效应表现为明显的整流和光电效应。我们的实验结果和建模表明,这些突出效应与中间温度下拓扑表面态(TSS)的空间不均匀形成密切相关。这项研究提供了一种打破镜像对称性(以及反转对称性)的方法,从而在金属拓扑表面态水坑之间形成 pn 结。这种效应为在低温下工作在射频范围内的高效电流整流器或能量收集设备铺平了道路,而利用其他具有大体隙的拓扑绝缘体,这种效应还可以扩展到高温。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
求助全文
约1分钟内获得全文 求助全文
来源期刊
CiteScore
19.00
自引率
0.90%
发文量
3575
审稿时长
2.5 months
期刊介绍: The Proceedings of the National Academy of Sciences (PNAS), a peer-reviewed journal of the National Academy of Sciences (NAS), serves as an authoritative source for high-impact, original research across the biological, physical, and social sciences. With a global scope, the journal welcomes submissions from researchers worldwide, making it an inclusive platform for advancing scientific knowledge.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信