Long-term reanalysis, future scenarios and impacts of nitrogen deposition on northern European ecosystems including the Baltic Sea and the Scandinavian Mountains

IF 8 1区 环境科学与生态学 Q1 ENVIRONMENTAL SCIENCES
Camilla Andersson , Tinja Olenius , Helene Alpfjord Wylde , Elin Almroth-Rosell , Robert G. Björk , Mats P. Björkman , Filip Moldan , Magnuz Engardt
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Abstract

This study illustrates how a temporally consistent deposition reanalysis can be used 1/ as input data to ecosystem impact assessments, 2/ to understand past trends, and 3/ for validation of decadal to century-scale model scenarios. We have constructed a multi-decadal (1983–2013) reanalysis of nitrogen deposition (NDEP) to northern Europe, including the Baltic Sea and the Scandinavian Mountains, using a combination of observations and modelling. We expanded the period with an operational annual reanalysis applying chemistry transport modelling, resulting in a fused dataset using the MATCH Sweden system for the period 1983–2021, and compared this to multi-century model scenarios of nitrogen deposition.
Since the 1980s, NDEP has decreased until early 2010s in northern Europe including the Baltic Sea (by 32 %) and the Scandinavian Mountains (by 19 %). Present NDEP is on pair with the levels in the 1950s, after peaking in 1980–1990. We project continued decrease in oxidized NDEP until 2050, but still exceeding the pre-industrial levels. We also project an increase in reduced NDEP from present to mid-21st century, with stronger signal compared to previous estimates. This results in a weakening of the annual reduction of NDEP, stabilizing to the levels of the 1940s to 1950s by mid-21st century, resulting in approximately twice as high NDEP compared to pre-industrial times. The projected NDEP decrease will likely not be sufficient to avoid future effects on sensitive ecosystems. Thus, there is a need for continued efforts to further decrease nitrogen emissions to the atmosphere for protection of terrestrial and aquatic environments, not the least as ecosystems are under additional pressure of climate change and intensive management. The NDEP trends and levels in our model scenarios compare well to the reanalysis results (including fused observations).

Abstract Image

长期再分析、未来情景和氮沉降对北欧生态系统的影响,包括波罗的海和斯堪的纳维亚山脉
本研究说明了如何利用时间上一致的沉积物再分析,1/作为生态系统影响评估的输入数据,2/了解过去的趋势,3/验证十年至百年尺度的模型方案。我们利用观测和模拟相结合的方法,构建了北欧(包括波罗的海和斯堪的纳维亚山脉)氮沉降的十年期(1983-2013 年)再分析(NDEP)。我们通过应用化学迁移建模的运行年度再分析,扩展了这一时期,从而利用瑞典 MATCH 系统得到了 1983-2021 年期间的融合数据集,并将其与多世纪氮沉降模型情景进行了比较。目前的 NDEP 与 20 世纪 50 年代的水平相当,在 1980-1990 年期间达到峰值。我们预计氧化型 NDEP 在 2050 年前将继续下降,但仍将超过工业化前的水平。我们还预测,从现在到 21 世纪中期,还原型 NDEP 将增加,与之前的估计相比,信号更强。这导致 NDEP 逐年减少的趋势减弱,到 21 世纪中叶稳定在 20 世纪 40 年代至 50 年代的水平,使 NDEP 与工业化前相比高出约两倍。预计的 NDEP 降幅可能不足以避免未来对敏感生态系统的影响。因此,有必要继续努力,进一步减少大气中的氮排放量,以保护陆地和水生环境,尤其是在生态系统面临气候变化和集约化管理的额外压力时。我们的模型方案中的 NDEP 趋势和水平与再分析结果(包括融合观测结果)相比都很好。
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来源期刊
Science of the Total Environment
Science of the Total Environment 环境科学-环境科学
CiteScore
17.60
自引率
10.20%
发文量
8726
审稿时长
2.4 months
期刊介绍: The Science of the Total Environment is an international journal dedicated to scientific research on the environment and its interaction with humanity. It covers a wide range of disciplines and seeks to publish innovative, hypothesis-driven, and impactful research that explores the entire environment, including the atmosphere, lithosphere, hydrosphere, biosphere, and anthroposphere. The journal's updated Aims & Scope emphasizes the importance of interdisciplinary environmental research with broad impact. Priority is given to studies that advance fundamental understanding and explore the interconnectedness of multiple environmental spheres. Field studies are preferred, while laboratory experiments must demonstrate significant methodological advancements or mechanistic insights with direct relevance to the environment.
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