{"title":"High Hole Mobility van der Waals Junction Field-Effect Transistors Based on Te/GaAs for Multimode Photodetection and Logic Applications.","authors":"Fei Li, Jiang Zeng, Yiming Zhao, Lingyu Zhu, Yao Zhou, Zuyi Wang, Zhen Wang, Yuhan Zhang, Guoxin Liu, Jingxian Xiong, Wei Gao, Mengmeng Yang, Jingbo Li, Nengjie Huo, Yiming Sun","doi":"10.1021/acsami.5c00891","DOIUrl":null,"url":null,"abstract":"<p><p>Recently, interface scattering and low mobility have significantly impeded the performance of two-dimensional (2D) P-type transistors. 2D semiconductor tellurium (Te) has garnered significant interest owing to its unique atomic chain crystal structure, which confers ultrahigh hole mobility. van der Waals heterojunction enhances transistor performance by reducing scattering at the gate-channel interface, attributed to its high-quality interface. In this study, we present Te/gallium arsenide (GaAs) hybrid dimensional JFETs exhibiting sizable on-state currents, elevated transconductance, and mobility as high as 328.4 cm<sup>2</sup>V<sup>-1</sup>s<sup>-1</sup>. Achieving a low-power device, we lowered the threshold voltage from 1.9 to 1 V by modifying the carrier concentration of the gate. Furthermore, enhancing negative photoconductivity on the Te surface is achieved by tuning the depth of the channel depletion region, thereby achieving an enhanced negative photoconductivity mechanism with universal applicability. Based on this, a photodetector featuring both positive and negative photoconductivity and a photovoltaic effect was developed. The negative photoresponsivity and detectivity at 635 nm of the device are -64 AW<sup>-1</sup> and 1.41 × 10<sup>10</sup> Jones, respectively. Utilizing these properties, we develop Te/GaAs JFET-based logic gate circuits and single-point negative photoconductive imaging applications. This provides a potential research avenue for future logic circuits and optoelectronic devices.</p>","PeriodicalId":5,"journal":{"name":"ACS Applied Materials & Interfaces","volume":" ","pages":"18655-18665"},"PeriodicalIF":8.3000,"publicationDate":"2025-03-26","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Materials & Interfaces","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acsami.5c00891","RegionNum":2,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"2025/3/11 0:00:00","PubModel":"Epub","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Recently, interface scattering and low mobility have significantly impeded the performance of two-dimensional (2D) P-type transistors. 2D semiconductor tellurium (Te) has garnered significant interest owing to its unique atomic chain crystal structure, which confers ultrahigh hole mobility. van der Waals heterojunction enhances transistor performance by reducing scattering at the gate-channel interface, attributed to its high-quality interface. In this study, we present Te/gallium arsenide (GaAs) hybrid dimensional JFETs exhibiting sizable on-state currents, elevated transconductance, and mobility as high as 328.4 cm2V-1s-1. Achieving a low-power device, we lowered the threshold voltage from 1.9 to 1 V by modifying the carrier concentration of the gate. Furthermore, enhancing negative photoconductivity on the Te surface is achieved by tuning the depth of the channel depletion region, thereby achieving an enhanced negative photoconductivity mechanism with universal applicability. Based on this, a photodetector featuring both positive and negative photoconductivity and a photovoltaic effect was developed. The negative photoresponsivity and detectivity at 635 nm of the device are -64 AW-1 and 1.41 × 1010 Jones, respectively. Utilizing these properties, we develop Te/GaAs JFET-based logic gate circuits and single-point negative photoconductive imaging applications. This provides a potential research avenue for future logic circuits and optoelectronic devices.
期刊介绍:
ACS Applied Materials & Interfaces is a leading interdisciplinary journal that brings together chemists, engineers, physicists, and biologists to explore the development and utilization of newly-discovered materials and interfacial processes for specific applications. Our journal has experienced remarkable growth since its establishment in 2009, both in terms of the number of articles published and the impact of the research showcased. We are proud to foster a truly global community, with the majority of published articles originating from outside the United States, reflecting the rapid growth of applied research worldwide.