High-Performance Edge-Line Contact Memristors with In-Plane Solid–Liquid–Solid Grown Silicon Nanowires for Probabilistic Neuromorphic Computing

IF 15.8 1区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY
ACS Nano Pub Date : 2025-03-11 DOI:10.1021/acsnano.4c16583
Lei Yan, Yifei Zhang, Zhiyan Hu, Zongguang Liu, Junzhuan Wang, Linwei Yu
{"title":"High-Performance Edge-Line Contact Memristors with In-Plane Solid–Liquid–Solid Grown Silicon Nanowires for Probabilistic Neuromorphic Computing","authors":"Lei Yan, Yifei Zhang, Zhiyan Hu, Zongguang Liu, Junzhuan Wang, Linwei Yu","doi":"10.1021/acsnano.4c16583","DOIUrl":null,"url":null,"abstract":"Memristors have garnered increasing attention in neuromorphic computing hardware due to their resistive switching characteristics. However, achieving uniformity across devices and further miniaturization for large-scale arrays remain critical challenges. In this study, we demonstrate the scalable production of highly uniform, quasi-one-dimensional diffusive memristors based on heavily doped n-type silicon nanowires (SiNWs) with diameters as small as ∼50 nm, fabricated via in-plane solid–liquid–solid (IPSLS) growth technology. The edge-line contact structural design improves the control of nucleation sites and the size of conductive filaments (CFs) in Ag/SiO<sub>2</sub>/n-SiNW memristors. These devices exhibit excellent self-compliance threshold switching characteristics, including a low operating voltage (∼0.8 V) with a standard deviation of 0.073 V, low leakage current (1 pA), high switching ratio (&gt;10<sup>7</sup>), ultrafast switching speed (∼8 ns), and extremely low switching energy (47.2 fJ per operation). Additionally, we developed neurons with tunable sigmoidal probabilistic activation functions, demonstrating high uniformity across different devices. These neurons achieved an accuracy of 96.2% in binary tumor classification tasks, underscoring the potential of IPSLS-fabricated SiNWs for advanced neuromorphic computing hardware. This work highlights the effectiveness of SiNW-based memristors in addressing challenges in neuromorphic hardware design and their potential for large-scale integration.","PeriodicalId":21,"journal":{"name":"ACS Nano","volume":"30 1","pages":""},"PeriodicalIF":15.8000,"publicationDate":"2025-03-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Nano","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acsnano.4c16583","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0

Abstract

Memristors have garnered increasing attention in neuromorphic computing hardware due to their resistive switching characteristics. However, achieving uniformity across devices and further miniaturization for large-scale arrays remain critical challenges. In this study, we demonstrate the scalable production of highly uniform, quasi-one-dimensional diffusive memristors based on heavily doped n-type silicon nanowires (SiNWs) with diameters as small as ∼50 nm, fabricated via in-plane solid–liquid–solid (IPSLS) growth technology. The edge-line contact structural design improves the control of nucleation sites and the size of conductive filaments (CFs) in Ag/SiO2/n-SiNW memristors. These devices exhibit excellent self-compliance threshold switching characteristics, including a low operating voltage (∼0.8 V) with a standard deviation of 0.073 V, low leakage current (1 pA), high switching ratio (>107), ultrafast switching speed (∼8 ns), and extremely low switching energy (47.2 fJ per operation). Additionally, we developed neurons with tunable sigmoidal probabilistic activation functions, demonstrating high uniformity across different devices. These neurons achieved an accuracy of 96.2% in binary tumor classification tasks, underscoring the potential of IPSLS-fabricated SiNWs for advanced neuromorphic computing hardware. This work highlights the effectiveness of SiNW-based memristors in addressing challenges in neuromorphic hardware design and their potential for large-scale integration.

Abstract Image

求助全文
约1分钟内获得全文 求助全文
来源期刊
ACS Nano
ACS Nano 工程技术-材料科学:综合
CiteScore
26.00
自引率
4.10%
发文量
1627
审稿时长
1.7 months
期刊介绍: ACS Nano, published monthly, serves as an international forum for comprehensive articles on nanoscience and nanotechnology research at the intersections of chemistry, biology, materials science, physics, and engineering. The journal fosters communication among scientists in these communities, facilitating collaboration, new research opportunities, and advancements through discoveries. ACS Nano covers synthesis, assembly, characterization, theory, and simulation of nanostructures, nanobiotechnology, nanofabrication, methods and tools for nanoscience and nanotechnology, and self- and directed-assembly. Alongside original research articles, it offers thorough reviews, perspectives on cutting-edge research, and discussions envisioning the future of nanoscience and nanotechnology.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
确定
请完成安全验证×
copy
已复制链接
快去分享给好友吧!
我知道了
右上角分享
点击右上角分享
0
联系我们:info@booksci.cn Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。 Copyright © 2023 布克学术 All rights reserved.
京ICP备2023020795号-1
ghs 京公网安备 11010802042870号
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术官方微信