Wenchao Li , Chen Guo , Meng Han , Minghui Tang , Chiheng Dong , Chao Yao , Dongliang Wang , Yanwei Ma
{"title":"Microstructural evolution mechanism of Ba0.6KαFe2As2 Cu/Ag composite sheathed superconducting tapes","authors":"Wenchao Li , Chen Guo , Meng Han , Minghui Tang , Chiheng Dong , Chao Yao , Dongliang Wang , Yanwei Ma","doi":"10.1016/j.supcon.2025.100154","DOIUrl":null,"url":null,"abstract":"<div><div>Low-cost Cu/Ag composite sheathed Ba<span><math><msub><mrow></mrow><mrow><mi>0.6</mi></mrow></msub></math></span>K<span><math><msub><mrow></mrow><mrow><mi>α</mi></mrow></msub></math></span>Fe<sub>2</sub>As<sub>2</sub> superconducting tapes have been the focus of considerable research interest in terms of superconducting properties and performance improvement. The K-doping content has a great influence on the transport critical current density (<span><math><msub><mrow><mi>J</mi></mrow><mrow><mi>c</mi></mrow></msub></math></span>) of Cu/Ag composite sheathed tapes. This study analyzes the evolution occurring within the micro-composition and the mechanism affecting the transport <span><math><msub><mrow><mi>J</mi></mrow><mrow><mi>c</mi></mrow></msub></math></span> in Ba<span><math><msub><mrow></mrow><mrow><mi>0.6</mi></mrow></msub></math></span>K<span><math><msub><mrow></mrow><mrow><mi>α</mi></mrow></msub></math></span>Fe<sub>2</sub>As<sub>2</sub> (0.42 <span><math><mo>≤</mo></math></span>\n <span><math><mi>α</mi></math></span>\n <span><math><mo>≤</mo></math></span> 0.54) raw material, by modulating the ratio of K. It has been demonstrated that both extremes of K content, namely an insufficient or excessive amount, have an adverse effect on phase purity of the powders. Consequently, this has a direct impact on the transport <span><math><msub><mrow><mi>J</mi></mrow><mrow><mi>c</mi></mrow></msub></math></span> of tapes. Cu/Ag tapes fabricated using a precursor powder with an optimal K ratio <span><math><mrow><mi>α</mi><mo>∼</mo></mrow></math></span>0.464 exhibited the highest performance, with a <span><math><msub><mrow><mi>J</mi></mrow><mrow><mi>c</mi></mrow></msub></math></span> of 5.8 × 10<sup>4</sup> A cm <sup>−2</sup> at 10 T and 4.2 K. The optimized Cu/Ag composite tapes have been found to have superior advantages for high-field applications.</div></div>","PeriodicalId":101185,"journal":{"name":"Superconductivity","volume":"13 ","pages":"Article 100154"},"PeriodicalIF":5.6000,"publicationDate":"2025-03-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Superconductivity","FirstCategoryId":"1085","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2772830725000055","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, ELECTRICAL & ELECTRONIC","Score":null,"Total":0}
引用次数: 0
Abstract
Low-cost Cu/Ag composite sheathed BaKFe2As2 superconducting tapes have been the focus of considerable research interest in terms of superconducting properties and performance improvement. The K-doping content has a great influence on the transport critical current density () of Cu/Ag composite sheathed tapes. This study analyzes the evolution occurring within the micro-composition and the mechanism affecting the transport in BaKFe2As2 (0.42
0.54) raw material, by modulating the ratio of K. It has been demonstrated that both extremes of K content, namely an insufficient or excessive amount, have an adverse effect on phase purity of the powders. Consequently, this has a direct impact on the transport of tapes. Cu/Ag tapes fabricated using a precursor powder with an optimal K ratio 0.464 exhibited the highest performance, with a of 5.8 × 104 A cm −2 at 10 T and 4.2 K. The optimized Cu/Ag composite tapes have been found to have superior advantages for high-field applications.