Shibin Deng, Heonjoon Park, Jonas Reimann, Jonas M. Peterson, Daria D. Blach, Meng-Jia Sun, Tengfei Yan, Dewei Sun, Takashi Taniguchi, Kenji Watanabe, Xiaodong Xu, Dante M. Kennes, Libai Huang
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引用次数: 0
Abstract
Moiré superlattices, such as those formed from transition metal dichalcogenide heterostructures, have emerged as an exciting platform for exploring quantum many-body physics. They have the potential to serve as solid-state analogues to ultracold gases for quantum simulations. A key open question is the coherence and dynamics of the quantum phases arising from photoexcited moiré excitons, particularly amid dissipation. Here we use transient photoluminescence and ultrafast reflectance microscopy to image non-equilibrium exciton phase transitions. Counterintuitively, experimental results and theoretical simulations indicate that strong long-range dipolar repulsion freezes the motion of the Mott insulator phase for over 70 ns. In mixed electron–exciton lattices, reduced dipolar interactions lead to diminished freezing dynamics. These findings challenge the prevailing notion that repulsion disperses particles, whereas attraction binds them. The observed phenomenon of frozen dynamics due to strong repulsive interactions is characteristic of highly coherent systems, a feature previously realized exclusively in ultracold gases. The authors image non-equilibrium exciton phase-transition dynamics in moiré superlattices, revealing how strong long-range dipolar repulsion freezes the motion of the Mott insulator over a timescale of tens of nanoseconds.
期刊介绍:
Nature Materials is a monthly multi-disciplinary journal aimed at bringing together cutting-edge research across the entire spectrum of materials science and engineering. It covers all applied and fundamental aspects of the synthesis/processing, structure/composition, properties, and performance of materials. The journal recognizes that materials research has an increasing impact on classical disciplines such as physics, chemistry, and biology.
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