Novel Field Experiment on Alkalinity Enhancement in Intertidal Environments—A Trailblazer for Natural Climate Solutions

IF 3.7 3区 环境科学与生态学 Q2 ENVIRONMENTAL SCIENCES
I. Mendes, J. Lübbers, J. Schönfeld, A. Baldermann, A. R. Carrasco, A. Cravo, A. Gomes, P. Grasse, F. M. Stamm
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Abstract

One recently proposed approach to reduce atmospheric CO2 concentrations is marine alkalinity enhancement. This technique increases the CO2 uptake capacity of seawater through weathering of fine-grained (mafic) rocks and minerals in marine environments. The weathering process has been extensively tested in laboratory studies and verified by numerical models. Field experiments scaling the CO2 uptake under natural conditions are still lacking. In a methodological approach, a novel in situ experiment was designed and installed in a salt marsh at Ria Formosa coastal lagoon, southern Portugal. The experiment comprised deployments of different sizes of olivine and basalt substrates, and a control site, which were tidally submerged twice a day. A monthly monitoring scheme of supernatant and porewater properties from each deployment and control site was established, and procedures for temperature, salinity, oxygen, pH, total alkalinity, nutrient, and trace metal analyses were defined. This paper is devoted to the methods and describes the design, a protocol for the analyses, and an evaluation of experimental performance and reliability. Data from the first 6 months are presented for validation of the experiment. They demonstrated elevated total alkalinity in water samples, mostly in porewater after the deployments, while salinity, oxygen, and pH reflect the control conditions. Significant alkalinity differences were observed between the treatments and the natural background conditions monitored at the control site, during the 6 months of the experiment. The methodological approach is presented with strengths, limitations, and recommendations for an upscaling as CO2 removal measure, servicing, and subsequent investigations.

Abstract Image

潮间带环境碱度增强的新野外试验——自然气候解决方案的先驱
最近提出的一种减少大气中二氧化碳浓度的方法是提高海洋的碱度。这项技术通过海洋环境中细粒(基性)岩石和矿物的风化作用,增加了海水对二氧化碳的吸收能力。风化过程已经在实验室研究中进行了广泛的测试,并通过数值模型进行了验证。在自然条件下衡量二氧化碳吸收的实地实验仍然缺乏。在方法论上,在葡萄牙南部Ria Formosa沿海泻湖的盐沼中设计并安装了一个新的原位实验。实验包括部署不同大小的橄榄石和玄武岩基质,以及一个对照地点,每天两次被潮汐淹没。建立了每个部署和控制点的上清液和孔隙水性质的月度监测方案,并定义了温度、盐度、氧、pH、总碱度、养分和痕量金属分析的程序。本文致力于方法和描述的设计,一个协议的分析,以及评估的实验性能和可靠性。提供前6个月的数据以验证实验。他们发现水样中的总碱度升高,主要是在部署后的孔隙水中,而盐度、氧气和pH值反映了控制条件。在6个月的试验期间,观察到处理与对照地点监测的自然背景条件之间存在显著的碱度差异。提出了该方法的优点、局限性,并提出了作为二氧化碳去除措施、服务和后续调查的升级建议。
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来源期刊
Journal of Geophysical Research: Biogeosciences
Journal of Geophysical Research: Biogeosciences Earth and Planetary Sciences-Paleontology
CiteScore
6.60
自引率
5.40%
发文量
242
期刊介绍: JGR-Biogeosciences focuses on biogeosciences of the Earth system in the past, present, and future and the extension of this research to planetary studies. The emerging field of biogeosciences spans the intellectual interface between biology and the geosciences and attempts to understand the functions of the Earth system across multiple spatial and temporal scales. Studies in biogeosciences may use multiple lines of evidence drawn from diverse fields to gain a holistic understanding of terrestrial, freshwater, and marine ecosystems and extreme environments. Specific topics within the scope of the section include process-based theoretical, experimental, and field studies of biogeochemistry, biogeophysics, atmosphere-, land-, and ocean-ecosystem interactions, biomineralization, life in extreme environments, astrobiology, microbial processes, geomicrobiology, and evolutionary geobiology
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