{"title":"Effect of Deposition Temperature on the Characteristics of Ga2O3 Films Grown on Flexible Mica and the Performance of Corresponding Photodetectors","authors":"Zhefeng Wang, Fabi Zhang*, Tangyou Sun, Xingpeng Liu, Ying Peng, Zanhui Chen, Peihua Wangyang, Daoyou Guo, Xu Wang and Haiou Li, ","doi":"10.1021/acsaom.4c0039410.1021/acsaom.4c00394","DOIUrl":null,"url":null,"abstract":"<p >In this study, we fabricated flexible Ga<sub>2</sub>O<sub>3</sub> photodetectors (PDs) based on Ga<sub>2</sub>O<sub>3</sub>/mica flexible structures obtained at different substrate temperatures. Higher substrate temperatures result in higher quality crystals for the film, but they also reduce the photoresponsivity of the PD. Meanwhile, the dark current of the PD gradually decreases, and the response time is significantly shortened. The PD fabricated at 440 °C exhibited a responsivity of 4.45 W/A at 20 V bias and weak UV illumination of approximately 380 μW/cm<sup>2</sup> (at 254 nm). It also demonstrated a high detectivity (<i>D</i>*) of 6.07 × 10<sup>12</sup> Jones and an extremely low noise equivalent power (NEP) of 4.42 × 10<sup>–13</sup> W/Hz<sup>1/2</sup>. At 680 °C, the PD exhibits an extremely low dark current (1.6 × 10<sup>–13</sup> A at 20 V) and a fast response time (τ<sub>rise</sub>: 0.89 s, τ<sub>decay</sub>: 0.26 s). Additionally, in bending tests, the PDs maintained nearly constant performance, demonstrating excellent flexibility and revealing the potential applications of Ga<sub>2</sub>O<sub>3</sub> flexible PDs in future wearable electronics.</p>","PeriodicalId":29803,"journal":{"name":"ACS Applied Optical Materials","volume":"3 2","pages":"272–283 272–283"},"PeriodicalIF":0.0000,"publicationDate":"2025-01-15","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"ACS Applied Optical Materials","FirstCategoryId":"1085","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acsaom.4c00394","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
引用次数: 0
Abstract
In this study, we fabricated flexible Ga2O3 photodetectors (PDs) based on Ga2O3/mica flexible structures obtained at different substrate temperatures. Higher substrate temperatures result in higher quality crystals for the film, but they also reduce the photoresponsivity of the PD. Meanwhile, the dark current of the PD gradually decreases, and the response time is significantly shortened. The PD fabricated at 440 °C exhibited a responsivity of 4.45 W/A at 20 V bias and weak UV illumination of approximately 380 μW/cm2 (at 254 nm). It also demonstrated a high detectivity (D*) of 6.07 × 1012 Jones and an extremely low noise equivalent power (NEP) of 4.42 × 10–13 W/Hz1/2. At 680 °C, the PD exhibits an extremely low dark current (1.6 × 10–13 A at 20 V) and a fast response time (τrise: 0.89 s, τdecay: 0.26 s). Additionally, in bending tests, the PDs maintained nearly constant performance, demonstrating excellent flexibility and revealing the potential applications of Ga2O3 flexible PDs in future wearable electronics.
期刊介绍:
ACS Applied Optical Materials is an international and interdisciplinary forum to publish original experimental and theoretical including simulation and modeling research in optical materials complementing the ACS Applied Materials portfolio. With a focus on innovative applications ACS Applied Optical Materials also complements and expands the scope of existing ACS publications that focus on fundamental aspects of the interaction between light and matter in materials science including ACS Photonics Macromolecules Journal of Physical Chemistry C ACS Nano and Nano Letters.The scope of ACS Applied Optical Materials includes high quality research of an applied nature that integrates knowledge in materials science chemistry physics optical science and engineering.