Accidental BICs and Chiroptical Response of Hollow Channels in Silicon Nanodisk Resonator-Based Metasurfaces for Chiral Sensing

Shubhanshi Sharma*, Alina Karabchevsky and Shailendra K. Varshney, 
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Abstract

Achieving light confinement at the nanoscale is essential for enhancing light-matter interactions, and bound states in the continuum (BICs) have emerged as promising approaches. This study presents a dielectric metasurface design featuring air channels within a silicon nanodisk resonator, demonstrating symmetry-protected BICs (SPBICs) and accidental BICs (ABICs). Here, we report SPBICs that exhibit an exceptionally high quality (Q) factor at very low asymmetry parameters. An increase in the asymmetry decreases the Q-factor quadratically. To alleviate this, we observe that the SPBIC can be transformed into ABICs by adjusting the radius of one air channel that converts the resonances from quasi-SPBICs to quasi-ABICs. Introducing a third air channel with an optimized radius helps to achieve an ultrahigh Q-factor ≈ 38000. Multiple ABICs with enhanced local fields were observed for both x- and y-polarizations. The triple air channel design also achieves a maximal extrinsic chiral response by breaking the symmetry through an oblique incidence angle, which influences circular dichroism (CD) and transmittance for different circular polarizations. Numerical simulations reveal that the proposed chiral metasurface achieves a near-perfect value of CD = −0.99, a Q-factor of 8846, and a field enhancement by a factor of 200. Moreover, slightly tilting the nanodisk can realize a high intrinsic chirality (CD = −0.88) with a Q-factor ≈ 104. The concept of chiral BICs studied here can be utilized in, but not limited to, applications such as chiral sensing, bioimaging, and chiroptical spectroscopy.

Abstract Image

基于硅纳米盘谐振器的手性传感超表面中空心通道的意外bic和手性响应
实现纳米尺度的光约束对于增强光与物质的相互作用至关重要,连续介质中的束缚态(bic)已经成为一种有前途的方法。本研究提出了一种在硅纳米盘谐振器中具有空气通道的介电超表面设计,展示了对称保护bic (spbic)和意外bic (ABICs)。在这里,我们报道了spbic在非常低的不对称参数下表现出非常高的质量(Q)因子。不对称性的增加会二次降低q因子。为了缓解这一问题,我们观察到,通过调整一个空气通道的半径,可以将SPBIC转换为ABICs,从而将准SPBIC转换为准ABICs。引入具有优化半径的第三个风道有助于实现超高q因子≈38000。在x极化和y极化下均观察到局部场增强的多个ABICs。三通道设计还通过斜入射角打破对称,实现了最大的外部手性响应,影响了圆二色性(CD)和不同圆偏振的透射率。数值模拟表明,所提出的手性超表面达到了近乎完美的CD = - 0.99, q因子为8846,场增强系数为200倍。此外,稍微倾斜的纳米盘可以实现高的本征手性(CD =−0.88),q因子≈104。本文所研究的手性bic概念可以应用于但不限于手性传感、生物成像和光谱学等应用。
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来源期刊
ACS Applied Optical Materials
ACS Applied Optical Materials 材料科学-光学材料-
CiteScore
1.10
自引率
0.00%
发文量
0
期刊介绍: ACS Applied Optical Materials is an international and interdisciplinary forum to publish original experimental and theoretical including simulation and modeling research in optical materials complementing the ACS Applied Materials portfolio. With a focus on innovative applications ACS Applied Optical Materials also complements and expands the scope of existing ACS publications that focus on fundamental aspects of the interaction between light and matter in materials science including ACS Photonics Macromolecules Journal of Physical Chemistry C ACS Nano and Nano Letters.The scope of ACS Applied Optical Materials includes high quality research of an applied nature that integrates knowledge in materials science chemistry physics optical science and engineering.
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