Advances in Membranes from Microporous Materials for Hydrogen Separation from Light Gases

IF 13 2区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY
Nicholaus Prasetya, I Gede Wenten, Bradley Paul Ladewig
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Abstract

With the pressing concern of the climate change, hydrogen will undoubtedly play an essential role in the future to accelerate the way out from fossil fuel-based economy. In this case, the role of membrane-based separation cannot be neglected since, compared with other conventional process, membrane-based process is more effective and consumes less energy. Regarding this, metal-based membranes, particularly palladium, are usually employed for hydrogen separation because of its high selectivity. However, with the advancement of various microporous materials, the status quo of the metal-based membranes could be challenged since, compared with the metal-based membranes, they could offer better hydrogen separation performance and could also be cheaper to be produced. In this article, the advancement of membranes fabricated from five main microporous materials, namely silica-based membranes, zeolite membranes, carbon-based membranes, metal organic frameworks/covalent organic frameworks (MOF/COF) membranes and microporous polymeric membranes, for hydrogen separation from light gases are extensively discussed. Their performances are then summarized to give further insights regarding the pathway that should be taken to direct the research direction in the future.

Abstract Image

轻气体氢分离用微孔材料膜研究进展
随着人们对气候变化的日益关注,氢无疑将在未来加速摆脱化石燃料经济的过程中发挥重要作用。在这种情况下,膜分离的作用不容忽视,因为与其他常规工艺相比,膜分离更有效,能耗更低。关于这一点,金属基膜,特别是钯基膜,由于其高选择性,通常用于氢分离。然而,随着各种微孔材料的进步,金属基膜的现状可能会受到挑战,因为与金属基膜相比,金属基膜可以提供更好的氢分离性能,而且生产成本也更低。本文对硅基膜、沸石膜、碳基膜、金属有机骨架/共价有机骨架(MOF/COF)膜和微孔聚合物膜等5种主要微孔材料制备的轻气体氢分离膜的研究进展进行了综述。然后对他们的表现进行总结,以进一步了解未来应该采取的指导研究方向的途径。
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来源期刊
Energy & Environmental Materials
Energy & Environmental Materials MATERIALS SCIENCE, MULTIDISCIPLINARY-
CiteScore
17.60
自引率
6.00%
发文量
66
期刊介绍: Energy & Environmental Materials (EEM) is an international journal published by Zhengzhou University in collaboration with John Wiley & Sons, Inc. The journal aims to publish high quality research related to materials for energy harvesting, conversion, storage, and transport, as well as for creating a cleaner environment. EEM welcomes research work of significant general interest that has a high impact on society-relevant technological advances. The scope of the journal is intentionally broad, recognizing the complexity of issues and challenges related to energy and environmental materials. Therefore, interdisciplinary work across basic science and engineering disciplines is particularly encouraged. The areas covered by the journal include, but are not limited to, materials and composites for photovoltaics and photoelectrochemistry, bioprocessing, batteries, fuel cells, supercapacitors, clean air, and devices with multifunctionality. The readership of the journal includes chemical, physical, biological, materials, and environmental scientists and engineers from academia, industry, and policy-making.
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