Hang Li, Bei Ding, Feng Zhou, Jie Chen, Linxuan Song, Wenyun Yang, Yong-Chang Lau, Jinbo Yang, Yue Li, Yong Jiang, Wenhong Wang
{"title":"Emergent Magnetic Skyrmions in a Topological Weyl Nodal Ring Semimetal","authors":"Hang Li, Bei Ding, Feng Zhou, Jie Chen, Linxuan Song, Wenyun Yang, Yong-Chang Lau, Jinbo Yang, Yue Li, Yong Jiang, Wenhong Wang","doi":"10.1021/acs.nanolett.4c06259","DOIUrl":null,"url":null,"abstract":"Topological magnetic materials are expected to show multiple transport responses because of their unusual bulk electronic topology in momentum space and their topological spin texture in real space. However, such multiple topological properties-hosting materials are rare in nature. In this work, we unambiguously reveal the emergence of magnetic skyrmions in Mn<sub>5</sub>Ge<sub>3</sub> single crystal through detailed electrical transport and Lorentz transmission electron microscopy (L-TEM) combined with <i>ab initio</i> calculations. We demonstrate that Mn<sub>5</sub>Ge<sub>3</sub> is a topological ferromagnet with multiple nodal rings in its electronic structure. Importantly, L-TEM experiments further reveal that the magnetic skyrmions appear in the (001) plane when an appropriate magnetic field is applied along the [001] direction. Skyrmion-induced topological Hall resistivity as large as ∼972 nΩ cm is also observed over a wide temperature-magnetic field region. These prove Mn<sub>5</sub>Ge<sub>3</sub> as a rare magnetic topological nodal-ring semimetal with great significance to explore novel topological multifunctionality, which facilitate the development of spintronics.","PeriodicalId":53,"journal":{"name":"Nano Letters","volume":"162 1","pages":""},"PeriodicalIF":9.6000,"publicationDate":"2025-02-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nano Letters","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1021/acs.nanolett.4c06259","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Topological magnetic materials are expected to show multiple transport responses because of their unusual bulk electronic topology in momentum space and their topological spin texture in real space. However, such multiple topological properties-hosting materials are rare in nature. In this work, we unambiguously reveal the emergence of magnetic skyrmions in Mn5Ge3 single crystal through detailed electrical transport and Lorentz transmission electron microscopy (L-TEM) combined with ab initio calculations. We demonstrate that Mn5Ge3 is a topological ferromagnet with multiple nodal rings in its electronic structure. Importantly, L-TEM experiments further reveal that the magnetic skyrmions appear in the (001) plane when an appropriate magnetic field is applied along the [001] direction. Skyrmion-induced topological Hall resistivity as large as ∼972 nΩ cm is also observed over a wide temperature-magnetic field region. These prove Mn5Ge3 as a rare magnetic topological nodal-ring semimetal with great significance to explore novel topological multifunctionality, which facilitate the development of spintronics.
期刊介绍:
Nano Letters serves as a dynamic platform for promptly disseminating original results in fundamental, applied, and emerging research across all facets of nanoscience and nanotechnology. A pivotal criterion for inclusion within Nano Letters is the convergence of at least two different areas or disciplines, ensuring a rich interdisciplinary scope. The journal is dedicated to fostering exploration in diverse areas, including:
- Experimental and theoretical findings on physical, chemical, and biological phenomena at the nanoscale
- Synthesis, characterization, and processing of organic, inorganic, polymer, and hybrid nanomaterials through physical, chemical, and biological methodologies
- Modeling and simulation of synthetic, assembly, and interaction processes
- Realization of integrated nanostructures and nano-engineered devices exhibiting advanced performance
- Applications of nanoscale materials in living and environmental systems
Nano Letters is committed to advancing and showcasing groundbreaking research that intersects various domains, fostering innovation and collaboration in the ever-evolving field of nanoscience and nanotechnology.