Technical, economic and lifecycle greenhouse gas emissions analyses of solid sorbent direct air capture technologies

Sylvanus Lilonfe , Sarah Rodgers , Amir F.N. Abdul-Manan , Ioanna Dimitriou , Jon McKechnie
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Abstract

Achieving net zero emissions by 2050 will require the development of cost-effective and CO2-efficient direct air capture (DAC) technology to remove atmospheric CO2. This study presents a comprehensive assessment of five solid sorbents under different technology scenarios to determine the design, operations, cost and greenhouse gas (GHG) emissions of DAC technologies. The cost and GHG emissions of the five solid sorbents ranged from $20241,200–40,400/t sorbent and 3.1–12.3 tCO2e/t sorbent in 2024, respectively, mainly driven by the raw materials used for sorbent manufacture. Cost estimates for the best capture technologies ranged from $202497–168/gross tCO2 captured [$2024126–170/net tCO2 captured] in 2025 and can be further reduced to $202487–140/gross tCO2 captured [$202493–142/net tCO2 captured] in 2050. The costs of DAC are heavily influenced by: (i) economic factors (i.e. capital expenses and energy costs), (ii) design elements (i.e. plant scale) and (iii) technical parameters (i.e. sorbent's adsorption rate and time). Conversely, the GHG emissions of DAC are mostly determined by the source of energy. Price signals in existing carbon markets are inadequate to support a DAC project, but a forecasted carbon price increase to $140–240/tCO2 by 2030–2050 could make DAC commercially viable.

Abstract Image

固体吸附剂直接空气捕获技术的技术、经济和生命周期温室气体排放分析
到2050年实现净零排放将需要开发成本效益高、二氧化碳效率高的直接空气捕获(DAC)技术来去除大气中的二氧化碳。本研究对五种不同技术方案下的固体吸附剂进行了综合评估,以确定DAC技术的设计、操作、成本和温室气体(GHG)排放。2024年,5种固体吸附剂的成本和温室气体排放量分别在20241美元、200 - 40400美元/t和3.1-12.3吨co2e /t之间,主要受吸附剂制造所用原材料的驱动。最佳捕集技术的成本估计在2025年为202497-168美元/总捕集吨二氧化碳[2024126-170美元/净捕集吨二氧化碳],到2050年可进一步降至202487-140美元/总捕集吨二氧化碳[202493-142美元/净捕集吨二氧化碳]。DAC的成本受到以下因素的严重影响:(i)经济因素(即资本支出和能源成本),(ii)设计因素(即工厂规模)和(iii)技术参数(即吸附剂的吸附率和时间)。反之,DAC的温室气体排放量主要由能源来源决定。现有碳市场的价格信号不足以支持DAC项目,但预计到2030-2050年,碳价格将上涨至每吨二氧化碳140-240美元,这可能使DAC在商业上可行。
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