Impact of UC2, UC, UBC and UB2 target compositions on the release of fission products

IF 1.4 3区物理与天体物理 Q3 INSTRUMENTS & INSTRUMENTATION

Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms Pub Date : 2025-02-01 DOI:10.1016/j.nimb.2024.165600

Julien Guillot , Brigitte Roussière , Sandrine Tusseau-Nenez , Isabelle Deloncle , Martin Humenny , Matthieu Lebois , Jean-François Ledu , Jérome Roques , François Brisset

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引用次数: 0

Abstract

The release properties of 4 targets (UC₂, UC, UBC, UB₂) were measured for 11 elements (Kr, Sr, Ru, Sn, Sb, Te, I, Cs, Ba, La, and Ce) using an off-line technique. The crystal packing fraction and the size of the studied element play a key role in the release process. However, physicochemical properties are also involved, notably melting and boiling points in vacuum and the minimal oxidation state. Principal component analysis was used to investigate the interrelationships between the physicochemical properties of fission products (from Fe to Dy) and the observed releases, thereby enabling predictions to be made about the release properties of the four crystallic configurations for elements that are inaccessible in off-line experiments.

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来源期刊

Nuclear Instruments & Methods in Physics Research Section B-beam Interactions With Materials and Atoms 物理-核科学技术

CiteScore

2.80

自引率

7.70%

发文量

231

审稿时长

1.9 months

期刊介绍： Section B of Nuclear Instruments and Methods in Physics Research covers all aspects of the interaction of energetic beams with atoms, molecules and aggregate forms of matter. This includes ion beam analysis and ion beam modification of materials as well as basic data of importance for these studies. Topics of general interest include: atomic collisions in solids, particle channelling, all aspects of collision cascades, the modification of materials by energetic beams, ion implantation, irradiation - induced changes in materials, the physics and chemistry of beam interactions and the analysis of materials by all forms of energetic radiation. Modification by ion, laser and electron beams for the study of electronic materials, metals, ceramics, insulators, polymers and other important and new materials systems are included. Related studies, such as the application of ion beam analysis to biological, archaeological and geological samples as well as applications to solve problems in planetary science are also welcome. Energetic beams of interest include atomic and molecular ions, neutrons, positrons and muons, plasmas directed at surfaces, electron and photon beams, including laser treated surfaces and studies of solids by photon radiation from rotating anodes, synchrotrons, etc. In addition, the interaction between various forms of radiation and radiation-induced deposition processes are relevant.