Tomohiro Nozaki , Xiaozhong Chen , Dae-Yeong Kim , Hyun-Ha Kim
{"title":"Plasma fluidized beds and their scalability","authors":"Tomohiro Nozaki , Xiaozhong Chen , Dae-Yeong Kim , Hyun-Ha Kim","doi":"10.1016/j.cogsc.2024.100984","DOIUrl":null,"url":null,"abstract":"<div><div>Over the last decade, plasma catalysis has attracted considerable research attention as an emerging low-carbon technology. In plasma catalysis, stable molecules such as CO<sub>2</sub>, CH<sub>4</sub>, and N<sub>2</sub> are activated by electron impact or electrical energy, thereby ushering in a low-temperature chemistry domain that departs from energy-intensive, heat-dependent systems. Moreover, renewable-energy-driven plasma technologies are expected to help realize power-to-X schemes. In this short review, fluidized bed (FB) reactors incorporated with dielectric barrier discharge (DBD) are explored as potential candidates for upscaling plasma catalysis systems without employing a numbering-up approach. To that end, a scaled-up FB-DBD reactor is conceptualized using CO<sub>2</sub> methanation as a model reaction, followed by the validation of laboratory-scale FB-DBD reactors, which exhibit remarkably high feed gas conversion rates at temperatures lower than those of thermal catalysis units. Finally, certain salient conclusions and perspectives are presented.</div></div>","PeriodicalId":54228,"journal":{"name":"Current Opinion in Green and Sustainable Chemistry","volume":"51 ","pages":"Article 100984"},"PeriodicalIF":9.3000,"publicationDate":"2025-02-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Current Opinion in Green and Sustainable Chemistry","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2452223624001056","RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Over the last decade, plasma catalysis has attracted considerable research attention as an emerging low-carbon technology. In plasma catalysis, stable molecules such as CO2, CH4, and N2 are activated by electron impact or electrical energy, thereby ushering in a low-temperature chemistry domain that departs from energy-intensive, heat-dependent systems. Moreover, renewable-energy-driven plasma technologies are expected to help realize power-to-X schemes. In this short review, fluidized bed (FB) reactors incorporated with dielectric barrier discharge (DBD) are explored as potential candidates for upscaling plasma catalysis systems without employing a numbering-up approach. To that end, a scaled-up FB-DBD reactor is conceptualized using CO2 methanation as a model reaction, followed by the validation of laboratory-scale FB-DBD reactors, which exhibit remarkably high feed gas conversion rates at temperatures lower than those of thermal catalysis units. Finally, certain salient conclusions and perspectives are presented.
期刊介绍:
The Current Opinion journals address the challenge specialists face in keeping up with the expanding information in their fields. In Current Opinion in Green and Sustainable Chemistry, experts present views on recent advances in a clear and readable form. The journal also provides evaluations of the most noteworthy papers, annotated by experts, from the extensive pool of original publications in Green and Sustainable Chemistry.