Ming-yu Shi, Ao Li, Tian-hao Ji, Da-jian Jv, Zhe-mi Xu
{"title":"Color change mechanism and application of oxidized carbon dots/I2O4 composite (OCDs/I2O4) in alcoholic beverages","authors":"Ming-yu Shi, Ao Li, Tian-hao Ji, Da-jian Jv, Zhe-mi Xu","doi":"10.1016/j.cartre.2024.100440","DOIUrl":null,"url":null,"abstract":"<div><div>Currently, ethanol detection in alcoholic beverages typically relies on complicated and costly approaches, including gas chromatography, liquid chromatography, and mass spectrometry, etc. Herein, we developed a non-toxicity, practical, low-cost and portable visual indicator for ethanol detection based on OCDs/I<sub>2</sub>O<sub>4</sub> nanopowders. By color change, the OCDs/I<sub>2</sub>O<sub>4</sub> can visually indicate ethanol concentration ranging from 14 % vol to 56 % vol and the detection limit can be further extended to 2 % vol with a UV-visible spectrum. The OCDs/I<sub>2</sub>O<sub>4</sub> indicator shows good stability and long-term endurance for at least 18 months, and it can be used under different temperatures (at least from 3 °C to 40 °C) and humidity (at least from 10 % to 90 %). A possible mechanism for the color change has been proposed based on the covalent-link hydrogen bonding change between OCDs and I<sub>2</sub>O<sub>4</sub>. The proposed OCDs/I<sub>2</sub>O<sub>4</sub> composite offers a convenient and practical solution for ethanol monitoring in various alcoholic beverages.</div></div>","PeriodicalId":52629,"journal":{"name":"Carbon Trends","volume":"18 ","pages":"Article 100440"},"PeriodicalIF":3.1000,"publicationDate":"2025-01-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Carbon Trends","FirstCategoryId":"1085","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2667056924001196","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Currently, ethanol detection in alcoholic beverages typically relies on complicated and costly approaches, including gas chromatography, liquid chromatography, and mass spectrometry, etc. Herein, we developed a non-toxicity, practical, low-cost and portable visual indicator for ethanol detection based on OCDs/I2O4 nanopowders. By color change, the OCDs/I2O4 can visually indicate ethanol concentration ranging from 14 % vol to 56 % vol and the detection limit can be further extended to 2 % vol with a UV-visible spectrum. The OCDs/I2O4 indicator shows good stability and long-term endurance for at least 18 months, and it can be used under different temperatures (at least from 3 °C to 40 °C) and humidity (at least from 10 % to 90 %). A possible mechanism for the color change has been proposed based on the covalent-link hydrogen bonding change between OCDs and I2O4. The proposed OCDs/I2O4 composite offers a convenient and practical solution for ethanol monitoring in various alcoholic beverages.