Bottom-Up Passivation Strategies toward High-Efficiency Carbon-Based All-Inorganic CsPbBr3 Perovskite Solar Cells

IF 9.6 1区化学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY

ACS Materials Letters Pub Date : 2024-11-29 DOI:10.1021/acsmaterialslett.4c0189010.1021/acsmaterialslett.4c01890

Mengjia Sui, Jiaojiao Zhang, Long Zhou*, Haonan Wu, Zhenhua Lin, Peixian Li*, Jincheng Zhang, Yue Hao and Jingjing Chang*,

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Abstract

Perovskite solar cells (PSCs) have been considered the next-generation star of the photovoltaic industry due to their high efficiency and significant application prospects. They are expected to break the Shockley–Quieisser limit of single-junction Si solar cells and promote the industrialization process of perovskites. All-inorganic CsPbBr₃ perovskites have received extensive attention due to their excellent photovoltaic properties and outstanding stability. Our work comprehensively reviews the recent progress of carbon-based CsPbBr₃ PSCs and systematically discusses the modified strategies to achieve high-performance CsPbBr₃ PSCs. Beginning with the CsPbBr₃ film preparation, we summarize the various optimization strategies for perovskite films regarding buried interface modification, additive passivation, and surface defect passivation. Moreover, the modifications of carbon electrodes are summarized and prospectively aimed at obtaining high efficiency. Finally, we discuss the recent advancements and challenges associated with carbon-based all-inorganic CsPbBr₃ PSCs.

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来源期刊

ACS Materials Letters MATERIALS SCIENCE, MULTIDISCIPLINARY-

CiteScore

14.60

自引率

3.50%

发文量

261

期刊介绍： ACS Materials Letters is a journal that publishes high-quality and urgent papers at the forefront of fundamental and applied research in the field of materials science. It aims to bridge the gap between materials and other disciplines such as chemistry, engineering, and biology. The journal encourages multidisciplinary and innovative research that addresses global challenges. Papers submitted to ACS Materials Letters should clearly demonstrate the need for rapid disclosure of key results. The journal is interested in various areas including the design, synthesis, characterization, and evaluation of emerging materials, understanding the relationships between structure, property, and performance, as well as developing materials for applications in energy, environment, biomedical, electronics, and catalysis. The journal has a 2-year impact factor of 11.4 and is dedicated to publishing transformative materials research with fast processing times. The editors and staff of ACS Materials Letters actively participate in major scientific conferences and engage closely with readers and authors. The journal also maintains an active presence on social media to provide authors with greater visibility.