Guifen Sun, Zhendong Sun, Peng Wang, Zhengyan Zhang, Chuizhou Meng, Shijie Guo, Yang Li
{"title":"Breathable, hydrophobic and antibacterial bioinspired fabric pressure sensors for comfortable skin-mountable health monitoring","authors":"Guifen Sun, Zhendong Sun, Peng Wang, Zhengyan Zhang, Chuizhou Meng, Shijie Guo, Yang Li","doi":"10.1016/j.cej.2025.159808","DOIUrl":null,"url":null,"abstract":"The development of flexible pressure sensors has attracted significant attention because of their critical role in wearable human health monitoring. However, most flexible sensors are constructed on impermeable polymer substrates, which cause an uncomfortable wearing experience owing to poor biocompatibility and breathability. Inspired by the advantages of natural Agropyron cristatum and octopuses, a flexible, breathable, hydrophobic, and antibacterial pressure sensor based on a permeable fabric platform is developed. The device is designed by sandwiching a microstructured gel ionic electrolyte between two zeolitic imidazolate frameworks-67 (ZIF-67)/silver nanowires (Ag NWs)/stearic acid (STA) fabric electrodes. Owing to the enhanced double-layer capacitive effect between the microstructured electrode–electrolyte interfaces, the sensor achieves outstanding sensitivity (∼751.57 kPa<sup>−1</sup>) and a wide detection range (∼84 kPa) with excellent durability. The micropores in the interior of the sensor provide good air permeability (∼350 mm s<sup>−1</sup>), and the STA nanosheets on the outside of the sensor exhibit hydrophobicity (contact angle ∼ 164.2°). Additionally, unique antibacterial ability is obtained by incorporating Ag NWs into ZIF-67. Consequently, a breathable and biocompatible wearing experience for the skin is achieved with sweatproof protection. The proposed strategy will render e-skins more comfortable, offering a favorable pathway for health monitoring.","PeriodicalId":270,"journal":{"name":"Chemical Engineering Journal","volume":"3 1","pages":""},"PeriodicalIF":13.3000,"publicationDate":"2025-01-22","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Chemical Engineering Journal","FirstCategoryId":"5","ListUrlMain":"https://doi.org/10.1016/j.cej.2025.159808","RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, CHEMICAL","Score":null,"Total":0}
引用次数: 0
Abstract
The development of flexible pressure sensors has attracted significant attention because of their critical role in wearable human health monitoring. However, most flexible sensors are constructed on impermeable polymer substrates, which cause an uncomfortable wearing experience owing to poor biocompatibility and breathability. Inspired by the advantages of natural Agropyron cristatum and octopuses, a flexible, breathable, hydrophobic, and antibacterial pressure sensor based on a permeable fabric platform is developed. The device is designed by sandwiching a microstructured gel ionic electrolyte between two zeolitic imidazolate frameworks-67 (ZIF-67)/silver nanowires (Ag NWs)/stearic acid (STA) fabric electrodes. Owing to the enhanced double-layer capacitive effect between the microstructured electrode–electrolyte interfaces, the sensor achieves outstanding sensitivity (∼751.57 kPa−1) and a wide detection range (∼84 kPa) with excellent durability. The micropores in the interior of the sensor provide good air permeability (∼350 mm s−1), and the STA nanosheets on the outside of the sensor exhibit hydrophobicity (contact angle ∼ 164.2°). Additionally, unique antibacterial ability is obtained by incorporating Ag NWs into ZIF-67. Consequently, a breathable and biocompatible wearing experience for the skin is achieved with sweatproof protection. The proposed strategy will render e-skins more comfortable, offering a favorable pathway for health monitoring.
期刊介绍:
The Chemical Engineering Journal is an international research journal that invites contributions of original and novel fundamental research. It aims to provide an international platform for presenting original fundamental research, interpretative reviews, and discussions on new developments in chemical engineering. The journal welcomes papers that describe novel theory and its practical application, as well as those that demonstrate the transfer of techniques from other disciplines. It also welcomes reports on carefully conducted experimental work that is soundly interpreted. The main focus of the journal is on original and rigorous research results that have broad significance. The Catalysis section within the Chemical Engineering Journal focuses specifically on Experimental and Theoretical studies in the fields of heterogeneous catalysis, molecular catalysis, and biocatalysis. These studies have industrial impact on various sectors such as chemicals, energy, materials, foods, healthcare, and environmental protection.