Catalytic Hydrogenation of CO2 by Direct Air Capture to Valuable C1 Products Using Homogenous Catalysts

IF 3.5 3区 化学 Q2 CHEMISTRY, MULTIDISCIPLINARY
Dr. Ritu Bhardwaj, Prof. Joyanta Choudhury
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引用次数: 0

Abstract

Growing atmospheric CO2 concentrations are a global concern and a primary factor contributing to global warming. Development of integrated CO2 capture and conversion protocols is necessary to mitigate this alarming challenge. Though CO2 hydrogenation to produce formic acid and methanol has seen many strides in the past decades, most studies utilize pure CO2 for this transformation. The CO2 concentration in the atmosphere stands at 400 ppm and reports that utilize direct air capture as the strategy to capture CO2 and utilize it for production of formic acid and methanol have only been reported in the past few years. This perspective summarizes such reports with a focus on the CO2-capturing additive, reaction solvent, and the molecular catalyst used to affect the transformation.

均相催化剂直接空气捕集法催化CO2加氢制取有价C1产品。
大气中二氧化碳浓度的增加是一个全球关注的问题,也是导致全球变暖的主要因素。为了缓解这一令人担忧的挑战,有必要制定综合的二氧化碳捕获和转换协议。虽然在过去的几十年里,二氧化碳加氢生产甲酸和甲醇已经取得了许多进展,但大多数研究都使用纯二氧化碳进行这种转化。大气中的二氧化碳浓度为400ppm,利用直接空气捕获作为捕获二氧化碳并利用其生产甲酸和甲醇的策略的报道仅在过去几年中才有报道。这一观点总结了这些报道,重点是二氧化碳捕获添加剂,反应溶剂,以及用于影响转化的分子催化剂。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
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来源期刊
Chemistry - An Asian Journal
Chemistry - An Asian Journal 化学-化学综合
CiteScore
7.00
自引率
2.40%
发文量
535
审稿时长
1.3 months
期刊介绍: Chemistry—An Asian Journal is an international high-impact journal for chemistry in its broadest sense. The journal covers all aspects of chemistry from biochemistry through organic and inorganic chemistry to physical chemistry, including interdisciplinary topics. Chemistry—An Asian Journal publishes Full Papers, Communications, and Focus Reviews. A professional editorial team headed by Dr. Theresa Kueckmann and an Editorial Board (headed by Professor Susumu Kitagawa) ensure the highest quality of the peer-review process, the contents and the production of the journal. Chemistry—An Asian Journal is published on behalf of the Asian Chemical Editorial Society (ACES), an association of numerous Asian chemical societies, and supported by the Gesellschaft Deutscher Chemiker (GDCh, German Chemical Society), ChemPubSoc Europe, and the Federation of Asian Chemical Societies (FACS).
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