pH-induced synergistic changes in color and shape of soft actuator based on degradable carbon dots/sodium alginate gel.

IF 10.7 1区 化学 Q1 CHEMISTRY, APPLIED
Carbohydrate Polymers Pub Date : 2025-03-01 Epub Date: 2024-12-06 DOI:10.1016/j.carbpol.2024.123112
Yingge Shi, Xuyuan Yang, Yongqiang Zhang, Siyu Lu
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引用次数: 0

Abstract

Soft actuators for intelligent robots require further elaboration to improve their biomedical applicability, which has led to the development of a series of flexible stimulus-responsive materials. However, fabricating degradable soft actuators that exhibit synergistic color and shape changes in response to environmental stimuli remains challenging. Here, we developed a soft actuating gel based on carbon dots (CDs) that are chemically cross-linked with sodium alginate. The soft actuating gel exhibits rapid synergistic changes in color and shape in response to pH owing to CDs protonation and deprotonation. Soft actuators constructed using the gel and poly (lactic acid) tape not only perform actions, such as grasping and lifting, but also camouflage and warn through self-color changes. The combination of pH-responsive CDs and degradable polymers provides a simple strategy for fabricating degradable soft actuators that exhibit synergistic changes in color and shape, and is expected to promote further research into soft actuators.

ph诱导的基于可降解碳点/海藻酸钠凝胶的软致动器颜色和形状的协同变化。
智能机器人的软执行器需要进一步完善,以提高其生物医学适用性,这导致了一系列柔性刺激响应材料的发展。然而,制造可降解的软致动器,在响应环境刺激时表现出协同的颜色和形状变化,仍然具有挑战性。在这里,我们开发了一种基于碳点(CDs)的软致动凝胶,它与海藻酸钠化学交联。由于CDs的质子化和去质子化,软致动凝胶在pH值下表现出快速的颜色和形状协同变化。使用凝胶和聚乳酸胶带构建的软致动器不仅可以执行抓取和抬起等动作,还可以通过自我颜色变化来伪装和警告。ph响应CDs和可降解聚合物的结合为制造可降解软致动器提供了一种简单的策略,可以在颜色和形状上产生协同变化,并有望促进软致动器的进一步研究。
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来源期刊
Carbohydrate Polymers
Carbohydrate Polymers 化学-高分子科学
CiteScore
22.40
自引率
8.00%
发文量
1286
审稿时长
47 days
期刊介绍: Carbohydrate Polymers stands as a prominent journal in the glycoscience field, dedicated to exploring and harnessing the potential of polysaccharides with applications spanning bioenergy, bioplastics, biomaterials, biorefining, chemistry, drug delivery, food, health, nanotechnology, packaging, paper, pharmaceuticals, medicine, oil recovery, textiles, tissue engineering, wood, and various aspects of glycoscience. The journal emphasizes the central role of well-characterized carbohydrate polymers, highlighting their significance as the primary focus rather than a peripheral topic. Each paper must prominently feature at least one named carbohydrate polymer, evident in both citation and title, with a commitment to innovative research that advances scientific knowledge.
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