MOF-derived Carbon-Based Materials for Energy-Related Applications

IF 27.4 1区材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY

Advanced Materials Pub Date : 2025-01-10 DOI:10.1002/adma.202413658

Lulu Chai, Rui Li, Yanzhi Sun, Kun Zhou, Junqing Pan

{"title":"MOF-derived Carbon-Based Materials for Energy-Related Applications","authors":"Lulu Chai, Rui Li, Yanzhi Sun, Kun Zhou, Junqing Pan","doi":"10.1002/adma.202413658","DOIUrl":null,"url":null,"abstract":"New carbon-based materials (CMs) are recommended as attractively active materials due to their diverse nanostructures and unique electron transport pathways, demonstrating great potential for highly efficient energy storage applications, electrocatalysis, and beyond. Among these newly reported CMs, metal–organic framework (MOF)-derived CMs have achieved impressive development momentum based on their high specific surface areas, tunable porosity, and flexible structural-functional integration. However, obstacles regarding the integrity of porous structures, the complexity of preparation processes, and the precise control of active components hinder the regulation of precise interface engineering in CMs. In this context, this review systematically summarizes the latest advances in tailored types, processing strategies, and energy-related applications of MOF-derived CMs and focuses on the structure-activity relationship of metal-free carbon, metal-doped carbon, and metallide-doped carbon. Particularly, the intrinsic correlation and evolutionary behavior between the synergistic interaction of micro/nanostructures and active species with electrochemical performances are emphasized. Finally, unique insights and perspectives on the latest relevant research are presented, and the future development prospects and challenges of MOF-derived CMs are discussed, providing valuable guidance to boost high-performance electrochemical electrodes for a broader range of application fields.","PeriodicalId":114,"journal":{"name":"Advanced Materials","volume":"36 1","pages":""},"PeriodicalIF":27.4000,"publicationDate":"2025-01-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advanced Materials","FirstCategoryId":"88","ListUrlMain":"https://doi.org/10.1002/adma.202413658","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}

引用次数: 0

Abstract

New carbon-based materials (CMs) are recommended as attractively active materials due to their diverse nanostructures and unique electron transport pathways, demonstrating great potential for highly efficient energy storage applications, electrocatalysis, and beyond. Among these newly reported CMs, metal–organic framework (MOF)-derived CMs have achieved impressive development momentum based on their high specific surface areas, tunable porosity, and flexible structural-functional integration. However, obstacles regarding the integrity of porous structures, the complexity of preparation processes, and the precise control of active components hinder the regulation of precise interface engineering in CMs. In this context, this review systematically summarizes the latest advances in tailored types, processing strategies, and energy-related applications of MOF-derived CMs and focuses on the structure-activity relationship of metal-free carbon, metal-doped carbon, and metallide-doped carbon. Particularly, the intrinsic correlation and evolutionary behavior between the synergistic interaction of micro/nanostructures and active species with electrochemical performances are emphasized. Finally, unique insights and perspectives on the latest relevant research are presented, and the future development prospects and challenges of MOF-derived CMs are discussed, providing valuable guidance to boost high-performance electrochemical electrodes for a broader range of application fields.

Abstract Image

查看原文本刊更多论文

求助全文

约1分钟内获得全文求助全文

来源期刊

Advanced Materials 工程技术-材料科学：综合

CiteScore

43.00

自引率

4.10%

发文量

2182

审稿时长

2 months

期刊介绍： Advanced Materials, one of the world's most prestigious journals and the foundation of the Advanced portfolio, is the home of choice for best-in-class materials science for more than 30 years. Following this fast-growing and interdisciplinary field, we are considering and publishing the most important discoveries on any and all materials from materials scientists, chemists, physicists, engineers as well as health and life scientists and bringing you the latest results and trends in modern materials-related research every week.