Lingling Sun, Yi Zeng, Jitao Li, Haoqi Wang, Qingsong Hua, Shun Lu
{"title":"Enhancing Water Electrolysis through Interfacial Design of Nickel Foam","authors":"Lingling Sun, Yi Zeng, Jitao Li, Haoqi Wang, Qingsong Hua, Shun Lu","doi":"10.1021/acs.langmuir.4c04714","DOIUrl":null,"url":null,"abstract":"Water electrolysis recognizes nickel foam (NF) as an effective current collector due to its excellent conductivity. However, recent studies highlighted NF’s effect on the efficacy of various electrocatalytic reactions, primarily due to the presence of electroactive chemical species at its interface. In contrast, numerous reports suggested that NF has a negligible impact on overall electrocatalytic activity. When evaluated against other current collectors, NF-supported catalysts demonstrate better electrochemical activity, predominantly due to NF’s interfacial design. This study presents an electrochemically relevant NF with a flexible interfacial design, supported by case studies and insights into promising future directions. This Perspective reveals the advantages, challenges, and overall applicability of NF’s interfacial design with the context of electrocatalytic water splitting in mind.","PeriodicalId":50,"journal":{"name":"Langmuir","volume":"57 1","pages":""},"PeriodicalIF":3.7000,"publicationDate":"2025-01-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":null,"platform":"Semanticscholar","paperid":null,"PeriodicalName":"Langmuir","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1021/acs.langmuir.4c04714","RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"CHEMISTRY, MULTIDISCIPLINARY","Score":null,"Total":0}
引用次数: 0
Abstract
Water electrolysis recognizes nickel foam (NF) as an effective current collector due to its excellent conductivity. However, recent studies highlighted NF’s effect on the efficacy of various electrocatalytic reactions, primarily due to the presence of electroactive chemical species at its interface. In contrast, numerous reports suggested that NF has a negligible impact on overall electrocatalytic activity. When evaluated against other current collectors, NF-supported catalysts demonstrate better electrochemical activity, predominantly due to NF’s interfacial design. This study presents an electrochemically relevant NF with a flexible interfacial design, supported by case studies and insights into promising future directions. This Perspective reveals the advantages, challenges, and overall applicability of NF’s interfacial design with the context of electrocatalytic water splitting in mind.
期刊介绍:
Langmuir is an interdisciplinary journal publishing articles in the following subject categories:
Colloids: surfactants and self-assembly, dispersions, emulsions, foams
Interfaces: adsorption, reactions, films, forces
Biological Interfaces: biocolloids, biomolecular and biomimetic materials
Materials: nano- and mesostructured materials, polymers, gels, liquid crystals
Electrochemistry: interfacial charge transfer, charge transport, electrocatalysis, electrokinetic phenomena, bioelectrochemistry
Devices and Applications: sensors, fluidics, patterning, catalysis, photonic crystals
However, when high-impact, original work is submitted that does not fit within the above categories, decisions to accept or decline such papers will be based on one criteria: What Would Irving Do?
Langmuir ranks #2 in citations out of 136 journals in the category of Physical Chemistry with 113,157 total citations. The journal received an Impact Factor of 4.384*.
This journal is also indexed in the categories of Materials Science (ranked #1) and Multidisciplinary Chemistry (ranked #5).